Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters

Kurzanzeige
dc.contributor.authorSenz, Volkmardeu
dc.contributor.authorFischer, Tim
dc.contributor.authorOelßner, Patricedeu
dc.contributor.authorTiggesbäumker, Josefdeu
dc.contributor.authorStanzel, Jörgdeu
dc.contributor.authorBostedt, Christophdeu
dc.contributor.authorThomas, Heikodeu
dc.contributor.authorSchöffler, Markusdeu
dc.contributor.authorFoucar, Lutzdeu
dc.contributor.authorMartins, Michaeldeu
dc.contributor.authorNeville, John J.deu
dc.contributor.authorNeeb, Matthiasdeu
dc.contributor.authorMöller, Thomasdeu
dc.contributor.authorWurth, Wilfrieddeu
dc.contributor.authorRühl, Eckartdeu
dc.contributor.authorDörner, Reinharddeu
dc.contributor.authorSchmidt-Böcking, Horstdeu
dc.contributor.authorEberhardt, Wolfgangdeu
dc.contributor.authorGanteför, Gerd
dc.contributor.authorTreusch, Rolfdeu
dc.contributor.authorRadcliffe, Pauldeu
dc.contributor.authorMeiwes-Broer, Karl-Heinzdeu
dc.date.accessioned2011-03-24T17:53:43Zdeu
dc.date.available2011-03-24T17:53:43Zdeu
dc.date.issued2009deu
dc.description.abstractMetal clusters serve as model systems to study basic problems of electronic correlation. Vacuum ultraviolet light from the free-electron laser FLASH ionizes 5d electrons from mass-separated negatively charged clusters, thus transiently leading to core-ionized neutral systems. Shielding of the core hole affects the electron binding energy. From the strong deviation from expectations of the metallic droplet and jellium models we conclude on reduced electronic shielding once the cluster size falls below about 20 atoms. This suggests a metal-to-nonmetal transition, in agreement with previous local density approximation calculations.eng
dc.description.versionpublished
dc.format.mimetypeapplication/pdfdeu
dc.identifier.citationFirst publ.in: Physical Review Letters 102 (2009), 138303deu
dc.identifier.doi10.1103/PhysRevLett.102.138303
dc.identifier.ppn310914043deu
dc.identifier.urihttp://kops.uni-konstanz.de/handle/123456789/9113
dc.language.isoengdeu
dc.legacy.dateIssued2009deu
dc.rightsterms-of-usedeu
dc.rights.urihttps://rightsstatements.org/page/InC/1.0/deu
dc.subject.ddc530deu
dc.subject.pacs73.22.-fdeu
dc.subject.pacs41.60.Crdeu
dc.subject.pacs36.20.Kddeu
dc.subject.pacs36.40.Eideu
dc.titleCore-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusterseng
dc.typeJOURNAL_ARTICLEdeu
dspace.entity.typePublication
kops.citation.bibtex
@article{Senz2009CoreH-9113,
  year={2009},
  doi={10.1103/PhysRevLett.102.138303},
  title={Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters},
  volume={102},
  journal={Physical Review Letters},
  author={Senz, Volkmar and Fischer, Tim and Oelßner, Patrice and Tiggesbäumker, Josef and Stanzel, Jörg and Bostedt, Christoph and Thomas, Heiko and Schöffler, Markus and Foucar, Lutz and Martins, Michael and Neville, John J. and Neeb, Matthias and Möller, Thomas and Wurth, Wilfried and Rühl, Eckart and Dörner, Reinhard and Schmidt-Böcking, Horst and Eberhardt, Wolfgang and Ganteför, Gerd and Treusch, Rolf and Radcliffe, Paul and Meiwes-Broer, Karl-Heinz},
  note={Article Number: 138303}
}
kops.citation.iso690SENZ, Volkmar, Tim FISCHER, Patrice OELSSNER, Josef TIGGESBÄUMKER, Jörg STANZEL, Christoph BOSTEDT, Heiko THOMAS, Markus SCHÖFFLER, Lutz FOUCAR, Michael MARTINS, John J. NEVILLE, Matthias NEEB, Thomas MÖLLER, Wilfried WURTH, Eckart RÜHL, Reinhard DÖRNER, Horst SCHMIDT-BÖCKING, Wolfgang EBERHARDT, Gerd GANTEFÖR, Rolf TREUSCH, Paul RADCLIFFE, Karl-Heinz MEIWES-BROER, 2009. Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters. In: Physical Review Letters. 2009, 102, 138303. Available under: doi: 10.1103/PhysRevLett.102.138303deu
kops.citation.iso690SENZ, Volkmar, Tim FISCHER, Patrice OELSSNER, Josef TIGGESBÄUMKER, Jörg STANZEL, Christoph BOSTEDT, Heiko THOMAS, Markus SCHÖFFLER, Lutz FOUCAR, Michael MARTINS, John J. NEVILLE, Matthias NEEB, Thomas MÖLLER, Wilfried WURTH, Eckart RÜHL, Reinhard DÖRNER, Horst SCHMIDT-BÖCKING, Wolfgang EBERHARDT, Gerd GANTEFÖR, Rolf TREUSCH, Paul RADCLIFFE, Karl-Heinz MEIWES-BROER, 2009. Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters. In: Physical Review Letters. 2009, 102, 138303. Available under: doi: 10.1103/PhysRevLett.102.138303eng
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