Publikation: Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters
Lade...
Dateien
Datum
2009
Autor:innen
Senz, Volkmar
Fischer, Tim
Oelßner, Patrice
Tiggesbäumker, Josef
Stanzel, Jörg
Bostedt, Christoph
Thomas, Heiko
Schöffler, Markus
Foucar, Lutz
Martins, Michael
Herausgeber:innen
ISSN der Zeitschrift
Electronic ISSN
ISBN
Bibliografische Daten
Verlag
Schriftenreihe
Auflagebezeichnung
URI (zitierfähiger Link)
DOI (zitierfähiger Link)
Internationale Patentnummer
Link zur Lizenz
Angaben zur Forschungsförderung
Projekt
Open Access-Veröffentlichung
Open Access Green
Sammlungen
Core Facility der Universität Konstanz
Titel in einer weiteren Sprache
Publikationstyp
Zeitschriftenartikel
Publikationsstatus
Published
Erschienen in
Physical Review Letters. 2009, 102, 138303. Available under: doi: 10.1103/PhysRevLett.102.138303
Zusammenfassung
Metal clusters serve as model systems to study basic problems of electronic correlation. Vacuum ultraviolet light from the free-electron laser FLASH ionizes 5d electrons from mass-separated negatively charged clusters, thus transiently leading to core-ionized neutral systems. Shielding of the core hole affects the electron binding energy. From the strong deviation from expectations of the metallic droplet and jellium models we conclude on reduced electronic shielding once the cluster size falls below about 20 atoms. This suggests a metal-to-nonmetal transition, in agreement with previous local density approximation calculations.
Zusammenfassung in einer weiteren Sprache
Fachgebiet (DDC)
530 Physik
Schlagwörter
Konferenz
Rezension
undefined / . - undefined, undefined
Zitieren
ISO 690
SENZ, Volkmar, Tim FISCHER, Patrice OELSSNER, Josef TIGGESBÄUMKER, Jörg STANZEL, Christoph BOSTEDT, Heiko THOMAS, Markus SCHÖFFLER, Lutz FOUCAR, Michael MARTINS, John J. NEVILLE, Matthias NEEB, Thomas MÖLLER, Wilfried WURTH, Eckart RÜHL, Reinhard DÖRNER, Horst SCHMIDT-BÖCKING, Wolfgang EBERHARDT, Gerd GANTEFÖR, Rolf TREUSCH, Paul RADCLIFFE, Karl-Heinz MEIWES-BROER, 2009. Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters. In: Physical Review Letters. 2009, 102, 138303. Available under: doi: 10.1103/PhysRevLett.102.138303BibTex
@article{Senz2009CoreH-9113,
year={2009},
doi={10.1103/PhysRevLett.102.138303},
title={Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters},
volume={102},
journal={Physical Review Letters},
author={Senz, Volkmar and Fischer, Tim and Oelßner, Patrice and Tiggesbäumker, Josef and Stanzel, Jörg and Bostedt, Christoph and Thomas, Heiko and Schöffler, Markus and Foucar, Lutz and Martins, Michael and Neville, John J. and Neeb, Matthias and Möller, Thomas and Wurth, Wilfried and Rühl, Eckart and Dörner, Reinhard and Schmidt-Böcking, Horst and Eberhardt, Wolfgang and Ganteför, Gerd and Treusch, Rolf and Radcliffe, Paul and Meiwes-Broer, Karl-Heinz},
note={Article Number: 138303}
}RDF
<rdf:RDF
xmlns:dcterms="http://purl.org/dc/terms/"
xmlns:dc="http://purl.org/dc/elements/1.1/"
xmlns:rdf="http://www.w3.org/1999/02/22-rdf-syntax-ns#"
xmlns:bibo="http://purl.org/ontology/bibo/"
xmlns:dspace="http://digital-repositories.org/ontologies/dspace/0.1.0#"
xmlns:foaf="http://xmlns.com/foaf/0.1/"
xmlns:void="http://rdfs.org/ns/void#"
xmlns:xsd="http://www.w3.org/2001/XMLSchema#" >
<rdf:Description rdf:about="https://kops.uni-konstanz.de/server/rdf/resource/123456789/9113">
<dc:creator>Neeb, Matthias</dc:creator>
<dspace:hasBitstream rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/9113/1/PhysRevLett102.pdf"/>
<dc:contributor>Ganteför, Gerd</dc:contributor>
<dcterms:abstract xml:lang="eng">Metal clusters serve as model systems to study basic problems of electronic correlation. Vacuum ultraviolet light from the free-electron laser FLASH ionizes 5d electrons from mass-separated negatively charged clusters, thus transiently leading to core-ionized neutral systems. Shielding of the core hole affects the electron binding energy. From the strong deviation from expectations of the metallic droplet and jellium models we conclude on reduced electronic shielding once the cluster size falls below about 20 atoms. This suggests a metal-to-nonmetal transition, in agreement with previous local density approximation calculations.</dcterms:abstract>
<dc:creator>Eberhardt, Wolfgang</dc:creator>
<dc:contributor>Dörner, Reinhard</dc:contributor>
<dc:creator>Oelßner, Patrice</dc:creator>
<dc:contributor>Rühl, Eckart</dc:contributor>
<dcterms:bibliographicCitation>First publ.in: Physical Review Letters 102 (2009), 138303</dcterms:bibliographicCitation>
<dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2011-03-24T17:53:43Z</dc:date>
<dc:creator>Martins, Michael</dc:creator>
<foaf:homepage rdf:resource="http://localhost:8080/"/>
<dc:creator>Radcliffe, Paul</dc:creator>
<dspace:isPartOfCollection rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/>
<dc:contributor>Neeb, Matthias</dc:contributor>
<dc:creator>Wurth, Wilfried</dc:creator>
<dc:contributor>Oelßner, Patrice</dc:contributor>
<dc:creator>Schmidt-Böcking, Horst</dc:creator>
<dc:creator>Ganteför, Gerd</dc:creator>
<dc:contributor>Radcliffe, Paul</dc:contributor>
<dc:creator>Dörner, Reinhard</dc:creator>
<dc:contributor>Wurth, Wilfried</dc:contributor>
<dc:contributor>Stanzel, Jörg</dc:contributor>
<dc:contributor>Meiwes-Broer, Karl-Heinz</dc:contributor>
<dcterms:isPartOf rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/>
<dc:contributor>Fischer, Tim</dc:contributor>
<dcterms:issued>2009</dcterms:issued>
<dc:contributor>Eberhardt, Wolfgang</dc:contributor>
<dc:contributor>Foucar, Lutz</dc:contributor>
<dc:creator>Möller, Thomas</dc:creator>
<void:sparqlEndpoint rdf:resource="http://localhost/fuseki/dspace/sparql"/>
<dc:contributor>Bostedt, Christoph</dc:contributor>
<dc:creator>Fischer, Tim</dc:creator>
<dc:contributor>Neville, John J.</dc:contributor>
<dc:format>application/pdf</dc:format>
<bibo:uri rdf:resource="http://kops.uni-konstanz.de/handle/123456789/9113"/>
<dc:creator>Bostedt, Christoph</dc:creator>
<dc:creator>Thomas, Heiko</dc:creator>
<dcterms:rights rdf:resource="https://rightsstatements.org/page/InC/1.0/"/>
<dc:contributor>Thomas, Heiko</dc:contributor>
<dc:contributor>Treusch, Rolf</dc:contributor>
<dc:creator>Stanzel, Jörg</dc:creator>
<dc:creator>Foucar, Lutz</dc:creator>
<dc:creator>Treusch, Rolf</dc:creator>
<dc:contributor>Schmidt-Böcking, Horst</dc:contributor>
<dc:creator>Meiwes-Broer, Karl-Heinz</dc:creator>
<dc:contributor>Martins, Michael</dc:contributor>
<dc:contributor>Senz, Volkmar</dc:contributor>
<dc:creator>Rühl, Eckart</dc:creator>
<dc:creator>Schöffler, Markus</dc:creator>
<dc:creator>Senz, Volkmar</dc:creator>
<dc:language>eng</dc:language>
<dcterms:title>Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters</dcterms:title>
<dc:contributor>Schöffler, Markus</dc:contributor>
<dc:contributor>Möller, Thomas</dc:contributor>
<dc:rights>terms-of-use</dc:rights>
<dc:contributor>Tiggesbäumker, Josef</dc:contributor>
<dc:creator>Tiggesbäumker, Josef</dc:creator>
<dc:creator>Neville, John J.</dc:creator>
<dcterms:available rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2011-03-24T17:53:43Z</dcterms:available>
<dcterms:hasPart rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/9113/1/PhysRevLett102.pdf"/>
</rdf:Description>
</rdf:RDF>Interner Vermerk
xmlui.Submission.submit.DescribeStep.inputForms.label.kops_note_fromSubmitter
Prüfungsdatum der Dissertation
Finanzierungsart
Kommentar zur Publikation
Allianzlizenz
Corresponding Authors der Uni Konstanz vorhanden
Internationale Co-Autor:innen
Universitätsbibliographie
Ja
