Publikation:

2D IR spectroscopy with phase-locked pulse pairs from a birefringent delay line

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Rehault_0-262159.pdf
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2014

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Rehault, Julien
Maiuri, Margherita
Manzoni, Cristian
Helbing, Jan
Cerullo, Giulio

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http://nbn-resolving.de/urn:nbn:de:bsz:352-0-262159
DOI (zitierfähiger Link)
https://doi.org/10.1364/OE.22.009063
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Physik: Publikationen
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Optics Express. 2014, 22(8), pp. 9063-9072. eISSN 1094-4087. Available under: doi: 10.1364/OE.22.009063

Zusammenfassung

We introduce a new scheme for two-dimensional IR spectroscopy in the partially collinear pump-probe geometry. Translating birefringent wedges allow generating phase-locked pump pulses with exceptional phase stability, in a simple and compact setup. A He-Ne tracking scheme permits to scan continuously the acquisition time. For a proof-of-principle demonstration we use lithium niobate, which allows operation up to 5 μm. Exploiting the inherent perpendicular polarizations of the two pump pulses, we also demonstrate signal enhancement and scattering suppression.

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ISO 690REHAULT, Julien, Margherita MAIURI, Cristian MANZONI, Daniele BRIDA, Jan HELBING, Giulio CERULLO, 2014. 2D IR spectroscopy with phase-locked pulse pairs from a birefringent delay line. In: Optics Express. 2014, 22(8), pp. 9063-9072. eISSN 1094-4087. Available under: doi: 10.1364/OE.22.009063
BibTex
@article{Rehault2014spect-29647,
  year={2014},
  doi={10.1364/OE.22.009063},
  title={2D IR spectroscopy with phase-locked pulse pairs from a birefringent delay line},
  number={8},
  volume={22},
  journal={Optics Express},
  pages={9063--9072},
  author={Rehault, Julien and Maiuri, Margherita and Manzoni, Cristian and Brida, Daniele and Helbing, Jan and Cerullo, Giulio}
}
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