2D IR spectroscopy with phase-locked pulse pairs from a birefringent delay line

Rehault, Julien; Maiuri, Margherita; Manzoni, Cristian; Brida, Daniele; Helbing, Jan; Cerullo, Giulio

2D IR spectroscopy with phase-locked pulse pairs from a birefringent delay line

Dateien

Rehault_0-262159.pdfGröße: 2.08 MBDownloads: 993

Datum

2014

Autor:innen

Rehault, Julien

Maiuri, Margherita

Manzoni, Cristian

Brida, Daniele

Helbing, Jan

Cerullo, Giulio

Open Access-Veröffentlichung

Open Access Gold

Sammlungen

Physik
Zukunftskolleg

Publikationstyp

Zeitschriftenartikel

Publikationsstatus

Published

Erschienen in

Optics Express. 2014, 22(8), pp. 9063-9072. eISSN 1094-4087. Available under: doi: 10.1364/OE.22.009063

Zusammenfassung

We introduce a new scheme for two-dimensional IR spectroscopy in the partially collinear pump-probe geometry. Translating birefringent wedges allow generating phase-locked pump pulses with exceptional phase stability, in a simple and compact setup. A He-Ne tracking scheme permits to scan continuously the acquisition time. For a proof-of-principle demonstration we use lithium niobate, which allows operation up to 5 μm. Exploiting the inherent perpendicular polarizations of the two pump pulses, we also demonstrate signal enhancement and scattering suppression.

Fachgebiet (DDC)

530 Physik

Zitieren

ISO 690

REHAULT, Julien, Margherita MAIURI, Cristian MANZONI, Daniele BRIDA, Jan HELBING, Giulio CERULLO, 2014. 2D IR spectroscopy with phase-locked pulse pairs from a birefringent delay line. In: Optics Express. 2014, 22(8), pp. 9063-9072. eISSN 1094-4087. Available under: doi: 10.1364/OE.22.009063

BibTex

@article{Rehault2014spect-29647,
  year={2014},
  doi={10.1364/OE.22.009063},
  title={2D IR spectroscopy with phase-locked pulse pairs from a birefringent delay line},
  number={8},
  volume={22},
  journal={Optics Express},
  pages={9063--9072},
  author={Rehault, Julien and Maiuri, Margherita and Manzoni, Cristian and Brida, Daniele and Helbing, Jan and Cerullo, Giulio}
}

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Universitätsbibliographie

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