Understanding enhanced rotational dynamics of active probes in rod suspensions

Thumbnail Image
Date
2022
Authors
Bos, Meike F.
Abaurrea-Velasco, Clara
de Graaf, Joost
Editors
Contact
Journal ISSN
Electronic ISSN
ISBN
Bibliographical data
Publisher
Series
DOI (citable link)
ArXiv-ID
International patent number
EU project number
693683
Project
Suspensions with Controlled Interaction Rules ASCIR
Open Access publication
Collections
Restricted until
Title in another language
Research Projects
Organizational Units
Journal Issue
Publication type
Journal article
Publication status
Published
Published in
Soft Matter ; 18 (2022), 33. - pp. 6246-6253. - Royal Society of Chemistry (RSC). - ISSN 1744-683X. - eISSN 1744-6848
Abstract
Active Brownian particles (APs) have recently been shown to exhibit enhanced rotational diffusion (ERD) in complex fluids. Here, we experimentally observe ERD and numerically corroborate its microscopic origin for a quasi-two-dimensional suspension of colloidal rods. At high density, the rods form small rafts, wherein they perform small-amplitude, high-frequency longitudinal displacements. Activity couples AP-rod contacts to reorientation, with the variance therein leading to ERD. This is captured by a local, rather than a global relaxation time, as used in previous phenomenological modeling. Our result should prove relevant to the microrheological characterization of complex fluids and furthering our understanding of the dynamics of microorganisms in such media.
Summary in another language
Subject (DDC)
530 Physics
Keywords
Conference
Review
undefined / . - undefined, undefined. - (undefined; undefined)
Cite This
ISO 690NARINDER, Narinder, Meike F. BOS, Clara ABAURREA-VELASCO, Joost DE GRAAF, Clemens BECHINGER, 2022. Understanding enhanced rotational dynamics of active probes in rod suspensions. In: Soft Matter. Royal Society of Chemistry (RSC). 18(33), pp. 6246-6253. ISSN 1744-683X. eISSN 1744-6848. Available under: doi: 10.1039/d2sm00583b
BibTex
@article{Narinder2022-08-24Under-58435,
  year={2022},
  doi={10.1039/d2sm00583b},
  title={Understanding enhanced rotational dynamics of active probes in rod suspensions},
  number={33},
  volume={18},
  issn={1744-683X},
  journal={Soft Matter},
  pages={6246--6253},
  author={Narinder, Narinder and Bos, Meike F. and Abaurrea-Velasco, Clara and de Graaf, Joost and Bechinger, Clemens}
}
RDF
<rdf:RDF
    xmlns:dcterms="http://purl.org/dc/terms/"
    xmlns:dc="http://purl.org/dc/elements/1.1/"
    xmlns:rdf="http://www.w3.org/1999/02/22-rdf-syntax-ns#"
    xmlns:bibo="http://purl.org/ontology/bibo/"
    xmlns:dspace="http://digital-repositories.org/ontologies/dspace/0.1.0#"
    xmlns:foaf="http://xmlns.com/foaf/0.1/"
    xmlns:void="http://rdfs.org/ns/void#"
    xmlns:xsd="http://www.w3.org/2001/XMLSchema#" > 
  <rdf:Description rdf:about="https://kops.uni-konstanz.de/server/rdf/resource/123456789/58435">
    <void:sparqlEndpoint rdf:resource="http://localhost/fuseki/dspace/sparql"/>
    <dcterms:available rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2022-08-30T13:57:19Z</dcterms:available>
    <dspace:isPartOfCollection rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/>
    <dc:creator>Narinder, Narinder</dc:creator>
    <dc:contributor>Bos, Meike F.</dc:contributor>
    <dcterms:rights rdf:resource="http://creativecommons.org/licenses/by-nc/3.0/"/>
    <dc:contributor>Narinder, Narinder</dc:contributor>
    <dc:contributor>Bechinger, Clemens</dc:contributor>
    <dc:rights>Attribution-NonCommercial 3.0 Unported</dc:rights>
    <foaf:homepage rdf:resource="http://localhost:8080/"/>
    <dcterms:title>Understanding enhanced rotational dynamics of active probes in rod suspensions</dcterms:title>
    <dcterms:issued>2022-08-24</dcterms:issued>
    <dcterms:hasPart rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/58435/1/Narinder_2-94c1cxxywrq9.pdf"/>
    <dc:contributor>de Graaf, Joost</dc:contributor>
    <dcterms:abstract xml:lang="eng">Active Brownian particles (APs) have recently been shown to exhibit enhanced rotational diffusion (ERD) in complex fluids. Here, we experimentally observe ERD and numerically corroborate its microscopic origin for a quasi-two-dimensional suspension of colloidal rods. At high density, the rods form small rafts, wherein they perform small-amplitude, high-frequency longitudinal displacements. Activity couples AP-rod contacts to reorientation, with the variance therein leading to ERD. This is captured by a local, rather than a global relaxation time, as used in previous phenomenological modeling. Our result should prove relevant to the microrheological characterization of complex fluids and furthering our understanding of the dynamics of microorganisms in such media.</dcterms:abstract>
    <dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2022-08-30T13:57:19Z</dc:date>
    <dspace:hasBitstream rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/58435/1/Narinder_2-94c1cxxywrq9.pdf"/>
    <dcterms:isPartOf rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/>
    <dc:creator>Abaurrea-Velasco, Clara</dc:creator>
    <dc:creator>Bechinger, Clemens</dc:creator>
    <dc:language>eng</dc:language>
    <bibo:uri rdf:resource="https://kops.uni-konstanz.de/handle/123456789/58435"/>
    <dc:contributor>Abaurrea-Velasco, Clara</dc:contributor>
    <dc:creator>de Graaf, Joost</dc:creator>
    <dc:creator>Bos, Meike F.</dc:creator>
  </rdf:Description>
</rdf:RDF>
Internal note
xmlui.Submission.submit.DescribeStep.inputForms.label.kops_note_fromSubmitter
Contact
URL of original publication
Test date of URL
Examination date of dissertation
Method of financing
Comment on publication
Alliance license
Corresponding Authors der Uni Konstanz vorhanden
International Co-Authors
Bibliography of Konstanz
Yes
Refereed
Yes