Femtosecond-resolved ablation dynamics of Si in the near field of a small dielectric particle
Femtosecond-resolved ablation dynamics of Si in the near field of a small dielectric particle
Date
2013
Authors
Puerto, Daniel
Garcia de Abajo, Francisco Javier
Siegel, Jan
Solis, Javier
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Beilstein Journal of Nanotechnology ; 4 (2013). - pp. 501-509. - eISSN 2190-4286
Abstract
In this work we analyze the ablation dynamics of crystalline Si in the intense near field generated by a small dielectric particle located at the material surface when being irradiated with an infrared femtosecond laser pulse (800 nm, 120 fs). The presence of the particle (7.9 μm diameter) leads to a strong local enhancement (ca. 40 times) of the incoming intensity of the pulse. The transient optical response of the material has been analyzed by means of fs-resolved optical microscopy in reflection configuration over a time span from 0.1 ps to about 1 ns. Characteristic phenomena like electron plasma formation, ultrafast melting and ablation, along with their characteristic time scales are observed in the region surrounding the particle. The use of a time resolved imaging technique allows us recording simultaneously the material response at ordinary and large peak power densities enabling a direct comparison between both scenarios. The time resolved images of near field exposed regions are consistent with a remarkable temporal shift of the ablation onset which occurs in the sub-picosend regime, from about 500 to 800 fs after excitation.
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530 Physics
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crystalline Si; fs-resolved microscopy; laser ablation; near-field enhancement; ultrafast dynamics
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KÜHLER, Paul, Daniel PUERTO, Mario MOSBACHER, Paul LEIDERER, Francisco Javier GARCIA DE ABAJO, Jan SIEGEL, Javier SOLIS, 2013. Femtosecond-resolved ablation dynamics of Si in the near field of a small dielectric particle. In: Beilstein Journal of Nanotechnology. 4, pp. 501-509. eISSN 2190-4286. Available under: doi: 10.3762/bjnano.4.59BibTex
@article{Kuhler2013Femto-42248, year={2013}, doi={10.3762/bjnano.4.59}, title={Femtosecond-resolved ablation dynamics of Si in the near field of a small dielectric particle}, volume={4}, journal={Beilstein Journal of Nanotechnology}, pages={501--509}, author={Kühler, Paul and Puerto, Daniel and Mosbacher, Mario and Leiderer, Paul and Garcia de Abajo, Francisco Javier and Siegel, Jan and Solis, Javier} }
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