Insights into optoelectronic properties of anti-solvent treated perovskite films

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NAWAZ, Asmat, Ali Koray ERDINC, Burak GULTEKIN, Muhammad TAYYIB, Ceylan ZAFER, Kaiying WANG, Ka Kan WONG, Sajad HUSSAIN, Lukas SCHMIDT-MENDE, Azhar FAKHARUDDIN, 2017. Insights into optoelectronic properties of anti-solvent treated perovskite films. In: Journal of Materials Science : Materials in Electronics. 28(20), pp. 15630-15636. ISSN 0957-4522. eISSN 1573-482X. Available under: doi: 10.1007/s10854-017-7451-z

@article{Nawaz2017-10Insig-40195, title={Insights into optoelectronic properties of anti-solvent treated perovskite films}, year={2017}, doi={10.1007/s10854-017-7451-z}, number={20}, volume={28}, issn={0957-4522}, journal={Journal of Materials Science : Materials in Electronics}, pages={15630--15636}, author={Nawaz, Asmat and Erdinc, Ali Koray and Gultekin, Burak and Tayyib, Muhammad and Zafer, Ceylan and Wang, Kaiying and Wong, Ka Kan and Hussain, Sajad and Schmidt-Mende, Lukas and Fakharuddin, Azhar} }

eng Wong, Ka Kan 2017-10 Fakharuddin, Azhar Erdinc, Ali Koray Insights into optoelectronic properties of anti-solvent treated perovskite films Tayyib, Muhammad 2017-09-28T14:44:05Z Wang, Kaiying Fakharuddin, Azhar Zafer, Ceylan Nawaz, Asmat Tayyib, Muhammad Wang, Kaiying Hussain, Sajad 2017-09-28T14:44:05Z Wong, Ka Kan Gultekin, Burak Schmidt-Mende, Lukas Hussain, Sajad Gultekin, Burak Schmidt-Mende, Lukas Nawaz, Asmat Erdinc, Ali Koray Zafer, Ceylan The remarkable performance in perovskite solar cells over the past few years primarily stemmed from an improvement in perovskite film composition and morphology. Antisolvent treatment of perovskite films is one such widely adopted method where a solvent other than that used for precursor solution is introduced to facilitate rapid crystallization of perovskite crystals and to obtain a homogeneous pin-hole free film. Various reports are published recently to understand solvent extraction mechanism, electrical properties and the effect of antisolvent treatment of perovskite film on device performance and stability. Herein, we report some more insights on the charge carrier dynamics, crystallinity and more importantly, the change in energy levels of antisolvent treated perovskite films. The UV–vis absorption, photoluminescence, and photoelectron spectroscopy measurements revealed a downward shift in energy levels of MAPbI<sub>3</sub> perovskite when treated with an antisolvent. The energy level shift favoured interfacial charge transfer and resulted in remarkable open-circuit voltage ~1.08 V and photoconversion efficiency 8.21% up from 0.61 V and 1.3% for a non-treated film, respectively for devices prepared at ambient conditions.

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