A Photoinduced Cyclization Cascade : Total Synthesis of (−)-Leuconoxine

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PFAFFENBACH, Magnus, Tanja GAICH, 2015. A Photoinduced Cyclization Cascade : Total Synthesis of (−)-Leuconoxine. In: Chemistry : a European journal. 21(17), pp. 6355-6357. ISSN 0947-6539. eISSN 1521-3765

@article{Pfaffenbach2015Photo-32755, title={A Photoinduced Cyclization Cascade : Total Synthesis of (−)-Leuconoxine}, year={2015}, doi={10.1002/chem.201500656}, number={17}, volume={21}, issn={0947-6539}, journal={Chemistry : a European journal}, pages={6355--6357}, author={Pfaffenbach, Magnus and Gaich, Tanja} }

<rdf:RDF xmlns:rdf="http://www.w3.org/1999/02/22-rdf-syntax-ns#" xmlns:bibo="http://purl.org/ontology/bibo/" xmlns:dc="http://purl.org/dc/elements/1.1/" xmlns:dcterms="http://purl.org/dc/terms/" xmlns:xsd="http://www.w3.org/2001/XMLSchema#" > <rdf:Description rdf:about="https://kops.uni-konstanz.de/rdf/resource/123456789/32755"> <dc:contributor>Pfaffenbach, Magnus</dc:contributor> <dc:contributor>Gaich, Tanja</dc:contributor> <dc:creator>Pfaffenbach, Magnus</dc:creator> <dcterms:available rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2016-01-28T14:30:17Z</dcterms:available> <dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2016-01-28T14:30:17Z</dc:date> <dcterms:abstract xml:lang="eng">A protecting-group-free and enantioselective total synthesis of the monoterpenoid indole alkaloid (-)-leuconoxine was accomplished. The key step comprises a novel photoinduced domino macrocyclization/transannular cyclization involving the Witkop cyclization, for which additional mechanistic evidence is provided. This process furnishes a diaza[5.5.6.6]fenestrane skeleton, which is a hitherto unprecedented structure element.</dcterms:abstract> <dcterms:title>A Photoinduced Cyclization Cascade : Total Synthesis of (−)-Leuconoxine</dcterms:title> <dcterms:issued>2015</dcterms:issued> <dc:language>eng</dc:language> <dc:creator>Gaich, Tanja</dc:creator> <bibo:uri rdf:resource="https://kops.uni-konstanz.de/handle/123456789/32755"/> </rdf:Description> </rdf:RDF>

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