Glass transition in a two-dimensional system of magnetic colloids
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We describe experiments on binary mixtures of superparamagnetic colloidal particles confined by gravity to a flat horizontal water-air interface. The colloids repel each other because of their magnetic dipole moments induced by a vertical external magnetic field B. By tuning B, the effective temperature of the system can be adjusted over several orders of magnitude. Particle coordinates are monitored by video-microscopy over more than five decades in time. Measured radial pair-distribution functions g(r) and mean-square displacements illustrate that this system is an ideal model of a two-dimensional (2D) glass former. We find that the effects of small amounts of aggregated particles only weakly affect the averaged structure and dynamics. Locally, a small number of elementary structural elements are observed each characterized by a special triangular shape. These triangles arrange in dense mostly space-filling arrays and account for the essential features of g(r). The long-time α-relaxation is related to drifts of arrays as well as erosion due to single particle and collective hopping events.
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KÖNIG, Hans, Klaus ZAHN, Georg MARET, 2004. Glass transition in a two-dimensional system of magnetic colloids. SLOW DYNAMICS IN COMPLEX SYSTEMS: 3rd International Symposium on Slow Dynamics in Complex Systems. Sendai (Japan). In: AIP Conference Proceedings. AIP, 2004, pp. 40-45. eISSN 0094-243X. Available under: doi: 10.1063/1.1764057BibTex
@inproceedings{Konig2004Glass-17296, year={2004}, doi={10.1063/1.1764057}, title={Glass transition in a two-dimensional system of magnetic colloids}, publisher={AIP}, booktitle={AIP Conference Proceedings}, pages={40--45}, author={König, Hans and Zahn, Klaus and Maret, Georg} }
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