Temperature Dependence of Hydrogen Adsorption Isotherms

dc.contributor.authorTibus, Stefan
dc.contributor.authorKlier, Jürgendeu
dc.contributor.authorLeiderer, Paul
dc.date.accessioned2011-03-24T17:55:09Zdeu
dc.date.available2011-03-24T17:55:09Zdeu
dc.date.issued2005deu
dc.description.abstractIn the past it has already been shown that adsorption isotherms of liquid or solid films are not described completely by the Frenkel-Halsey-Hill theory. Substrate roughness as well as thermal fluctuations have to be taken into account in understanding the adsorption behavior. The inclusion of thermal fluctuations into the adsorption theory has already been addressed and proven to provide an explanation for the deviations found in many experiments. However, a resulting temperature dependence of such isotherms has not yet been verifed. In our investigations we have addressed this issue with a series of adsorption isotherms of hydrogen on gold in a temperature range from 11K to 19.5K (i.e., below and above the triple-point temperature of hydrogen). Our measurements are compared with existing theories and the nature of the remaining discrepancies is discussed.eng
dc.description.versionpublished
dc.format.mimetypeapplication/pdfdeu
dc.identifier.citationFirst publ. in: Journal of Low Temperature Physics 139 (2005), 5-6, pp. 531-539deu
dc.identifier.doi10.1007/s10909-005-5440-8
dc.identifier.ppn264521838deu
dc.identifier.urihttp://kops.uni-konstanz.de/handle/123456789/9282
dc.language.isoengdeu
dc.legacy.dateIssued2007deu
dc.rightsAttribution-NonCommercial-NoDerivs 2.0 Generic
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/2.0/
dc.subject.ddc530deu
dc.titleTemperature Dependence of Hydrogen Adsorption Isothermseng
dc.typeJOURNAL_ARTICLEdeu
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  doi={10.1007/s10909-005-5440-8},
  title={Temperature Dependence of Hydrogen Adsorption Isotherms},
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  volume={139},
  journal={Journal of Low Temperature Physics},
  pages={531--539},
  author={Tibus, Stefan and Klier, Jürgen and Leiderer, Paul}
}
kops.citation.iso690TIBUS, Stefan, Jürgen KLIER, Paul LEIDERER, 2005. Temperature Dependence of Hydrogen Adsorption Isotherms. In: Journal of Low Temperature Physics. 2005, 139(5-6), pp. 531-539. Available under: doi: 10.1007/s10909-005-5440-8deu
kops.citation.iso690TIBUS, Stefan, Jürgen KLIER, Paul LEIDERER, 2005. Temperature Dependence of Hydrogen Adsorption Isotherms. In: Journal of Low Temperature Physics. 2005, 139(5-6), pp. 531-539. Available under: doi: 10.1007/s10909-005-5440-8eng
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