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Efficient nonlinear light emission of single gold optical antennas driven by few-cycle near-infrared pulses

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2009

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Träutlein, Daniel
Wild, Barbara

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http://nbn-resolving.de/urn:nbn:de:bsz:352-opus-107109
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https://doi.org/10.1103/PhysRevLett.103.257404
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Physical Review Letters. 2009, 103, 257404. Available under: doi: 10.1103/PhysRevLett.103.257404

Zusammenfassung

Individual nanometer-sized plasmonic antennas are excited resonantly with few-cycle laser pulses in the near infrared. Intense third-harmonic emission of visible light prevails for fundamental photon energies below 1.1 eV. Interband luminescence and second harmonic generation occur solely at higher driving frequencies. We attribute these findings to multiphoton resonances with the d-band transitions of gold. The strong third-order signal allows direct measurement of a subcycle plasmon dephasing time of 2 fs, highlighting the efficient radiation coupling and broadband response of the devices.

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ISO 690HANKE, Tobias, Günther KRAUSS, Daniel TRÄUTLEIN, Barbara WILD, Rudolf BRATSCHITSCH, Alfred LEITENSTORFER, 2009. Efficient nonlinear light emission of single gold optical antennas driven by few-cycle near-infrared pulses. In: Physical Review Letters. 2009, 103, 257404. Available under: doi: 10.1103/PhysRevLett.103.257404
BibTex
@article{Hanke2009Effic-889,
  year={2009},
  doi={10.1103/PhysRevLett.103.257404},
  title={Efficient nonlinear light emission of single gold optical antennas driven by few-cycle near-infrared pulses},
  volume={103},
  journal={Physical Review Letters},
  author={Hanke, Tobias and Krauss, Günther and Träutlein, Daniel and Wild, Barbara and Bratschitsch, Rudolf and Leitenstorfer, Alfred},
  note={Article Number: 257404}
}
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