Relaxation dynamics of the mass-​selected hydrated auride ion (Au-​)

dc.contributor.authorBraun, Christian
dc.contributor.authorPietsch, Susanne
dc.contributor.authorProch, Sebastian
dc.contributor.authorKim, Young Dokdeu
dc.contributor.authorGanteför, Gerd
dc.date.accessioned2014-03-04T09:56:33Zdeu
dc.date.available2014-03-04T09:56:33Zdeu
dc.date.issued2013
dc.description.abstractBy using time-​resolved photoelectron spectroscopy, decay of optically excited states of hydrated Au-​ mass-​selected in the gas phase was studied. Probably the pump-​photon can induce injection of an electron from auride chromophore to the H2O solvent. The cluster with 3 H2O mols. (Au-​(H2O)​3) showed a long-​living excited state with a lifetime of ∼19 ± 3 ps, whereas that of Au-​(H2O)​2 is only ∼3 ± 1 ps. The fate of an optically excited state of an ionic species can be significantly changed by the no. of H2O (solvent) mols. attached.eng
dc.description.versionpublished
dc.identifier.citationChemical Physics Letters ; 588 (2013). - S. 27-30deu
dc.identifier.doi10.1016/j.cplett.2013.09.064deu
dc.identifier.ppn411071602deu
dc.identifier.urihttp://kops.uni-konstanz.de/handle/123456789/26614
dc.language.isoengdeu
dc.legacy.dateIssued2014-03-04deu
dc.rightsterms-of-usedeu
dc.rights.urihttps://rightsstatements.org/page/InC/1.0/deu
dc.subjectpump-probe spectroscopydeu
dc.subjectsolvationdeu
dc.subjectgolddeu
dc.subject.ddc540deu
dc.titleRelaxation dynamics of the mass-​selected hydrated auride ion (Au<sup>-</sup>​)eng
dc.typeJOURNAL_ARTICLEdeu
dspace.entity.typePublication
kops.citation.bibtex
@article{Braun2013Relax-26614,
  year={2013},
  doi={10.1016/j.cplett.2013.09.064},
  title={Relaxation dynamics of the mass-​selected hydrated auride ion (Au<sup>-</sup>​)},
  volume={588},
  issn={0009-2614},
  journal={Chemical Physics Letters},
  pages={27--30},
  author={Braun, Christian and Pietsch, Susanne and Proch, Sebastian and Kim, Young Dok and Ganteför, Gerd},
  note={Erratum to ‘Relaxation dynamics... ': We included above the corrected author list. One of the co-authors, Susanne Pietsch, was missing in the originally published Letter. The main contributions from Susanne Pietsch were the photoelectron spectra of Au−(H2O)m with m = 0–6 shown in Figure 1 measured with a photon energy of 7.9 eV. These data were critical to understand the data of the femtosecond time-resolved photoelectron spectroscopy. [Chemical Physics Letters ; https://doi.org/10.1016/j.cplett.2014.01.032]}
}
kops.citation.iso690BRAUN, Christian, Susanne PIETSCH, Sebastian PROCH, Young Dok KIM, Gerd GANTEFÖR, 2013. Relaxation dynamics of the mass-​selected hydrated auride ion (Au-​). In: Chemical Physics Letters. 2013, 588, pp. 27-30. ISSN 0009-2614. eISSN 1873-4448. Available under: doi: 10.1016/j.cplett.2013.09.064deu
kops.citation.iso690BRAUN, Christian, Susanne PIETSCH, Sebastian PROCH, Young Dok KIM, Gerd GANTEFÖR, 2013. Relaxation dynamics of the mass-​selected hydrated auride ion (Au-​). In: Chemical Physics Letters. 2013, 588, pp. 27-30. ISSN 0009-2614. eISSN 1873-4448. Available under: doi: 10.1016/j.cplett.2013.09.064eng
kops.citation.rdf
<rdf:RDF
    xmlns:dcterms="http://purl.org/dc/terms/"
    xmlns:dc="http://purl.org/dc/elements/1.1/"
    xmlns:rdf="http://www.w3.org/1999/02/22-rdf-syntax-ns#"
    xmlns:bibo="http://purl.org/ontology/bibo/"
    xmlns:dspace="http://digital-repositories.org/ontologies/dspace/0.1.0#"
    xmlns:foaf="http://xmlns.com/foaf/0.1/"
    xmlns:void="http://rdfs.org/ns/void#"
    xmlns:xsd="http://www.w3.org/2001/XMLSchema#" > 
  <rdf:Description rdf:about="https://kops.uni-konstanz.de/server/rdf/resource/123456789/26614">
    <dcterms:title>Relaxation dynamics of the mass-​selected hydrated auride ion (Au&lt;sup&gt;-&lt;/sup&gt;​)</dcterms:title>
    <dcterms:rights rdf:resource="https://rightsstatements.org/page/InC/1.0/"/>
    <dc:creator>Kim, Young Dok</dc:creator>
    <dc:rights>terms-of-use</dc:rights>
    <dcterms:isPartOf rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/>
    <dc:creator>Proch, Sebastian</dc:creator>
    <dc:contributor>Kim, Young Dok</dc:contributor>
    <dc:contributor>Ganteför, Gerd</dc:contributor>
    <dspace:hasBitstream rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/26614/2/Braun_266146.pdf"/>
    <dc:contributor>Proch, Sebastian</dc:contributor>
    <dc:language>eng</dc:language>
    <dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2014-03-04T09:56:33Z</dc:date>
    <dc:creator>Pietsch, Susanne</dc:creator>
    <dcterms:available rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2014-03-04T09:56:33Z</dcterms:available>
    <dcterms:bibliographicCitation>Chemical Physics Letters ; 588 (2013). - S. 27-30</dcterms:bibliographicCitation>
    <dc:creator>Braun, Christian</dc:creator>
    <dcterms:hasPart rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/26614/2/Braun_266146.pdf"/>
    <dcterms:issued>2013</dcterms:issued>
    <void:sparqlEndpoint rdf:resource="http://localhost/fuseki/dspace/sparql"/>
    <dspace:isPartOfCollection rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/>
    <bibo:uri rdf:resource="http://kops.uni-konstanz.de/handle/123456789/26614"/>
    <dc:contributor>Pietsch, Susanne</dc:contributor>
    <dcterms:abstract xml:lang="eng">By using time-​resolved photoelectron spectroscopy, decay of optically excited states of hydrated Au-​ mass-​selected in the gas phase was studied.  Probably the pump-​photon can induce injection of an electron from auride chromophore to the H2O solvent.  The cluster with 3 H2O mols. (Au-​(H2O)​3) showed a long-​living excited state with a lifetime of ∼19 ± 3 ps, whereas that of Au-​(H2O)​2 is only ∼3 ± 1 ps.  The fate of an optically excited state of an ionic species can be significantly changed by the no. of H2O (solvent) mols. attached.</dcterms:abstract>
    <dc:creator>Ganteför, Gerd</dc:creator>
    <dc:contributor>Braun, Christian</dc:contributor>
    <foaf:homepage rdf:resource="http://localhost:8080/"/>
  </rdf:Description>
</rdf:RDF>
kops.description.commentErratum to ‘Relaxation dynamics... ': We included above the corrected author list. One of the co-authors, Susanne Pietsch, was missing in the originally published Letter. The main contributions from Susanne Pietsch were the photoelectron spectra of Au−(H2O)m with m = 0–6 shown in Figure 1 measured with a photon energy of 7.9 eV. These data were critical to understand the data of the femtosecond time-resolved photoelectron spectroscopy. [Chemical Physics Letters ; https://doi.org/10.1016/j.cplett.2014.01.032]deu
kops.description.openAccessopenaccessgreen
kops.flag.knbibliographytrue
kops.identifier.nbnurn:nbn:de:bsz:352-266146deu
kops.sourcefieldChemical Physics Letters. 2013, <b>588</b>, pp. 27-30. ISSN 0009-2614. eISSN 1873-4448. Available under: doi: 10.1016/j.cplett.2013.09.064deu
kops.sourcefield.plainChemical Physics Letters. 2013, 588, pp. 27-30. ISSN 0009-2614. eISSN 1873-4448. Available under: doi: 10.1016/j.cplett.2013.09.064deu
kops.sourcefield.plainChemical Physics Letters. 2013, 588, pp. 27-30. ISSN 0009-2614. eISSN 1873-4448. Available under: doi: 10.1016/j.cplett.2013.09.064eng
kops.submitter.emailsebastian.proch@uni-konstanz.dedeu
relation.isAuthorOfPublicationf217b1ab-7239-4c34-84b4-14287c922ba8
relation.isAuthorOfPublicationaa9f830e-3c67-4e5c-bb9a-5bf467c6e2a6
relation.isAuthorOfPublicationf0bc7b58-7a92-456e-80e9-a2d915c19db9
relation.isAuthorOfPublicationd81f0b28-9ec2-4bdb-b325-21714f128d3c
relation.isAuthorOfPublication.latestForDiscoveryf217b1ab-7239-4c34-84b4-14287c922ba8
source.bibliographicInfo.fromPage27
source.bibliographicInfo.toPage30
source.bibliographicInfo.volume588
source.identifier.eissn1873-4448deu
source.identifier.issn0009-2614
source.periodicalTitleChemical Physics Letters

Dateien

Originalbündel

Gerade angezeigt 1 - 1 von 1
Vorschaubild nicht verfügbar
Name:
Braun_266146.pdf
Größe:
595.05 KB
Format:
Adobe Portable Document Format
Braun_266146.pdf
Braun_266146.pdfGröße: 595.05 KBDownloads: 447

Lizenzbündel

Gerade angezeigt 1 - 1 von 1
Vorschaubild nicht verfügbar
Name:
license.txt
Größe:
1.92 KB
Format:
Plain Text
Beschreibung:
license.txt
license.txtGröße: 1.92 KBDownloads: 0