Relaxation dynamics of the mass-selected hydrated auride ion (Au-)
| dc.contributor.author | Braun, Christian | |
| dc.contributor.author | Pietsch, Susanne | |
| dc.contributor.author | Proch, Sebastian | |
| dc.contributor.author | Kim, Young Dok | deu |
| dc.contributor.author | Ganteför, Gerd | |
| dc.date.accessioned | 2014-03-04T09:56:33Z | deu |
| dc.date.available | 2014-03-04T09:56:33Z | deu |
| dc.date.issued | 2013 | |
| dc.description.abstract | By using time-resolved photoelectron spectroscopy, decay of optically excited states of hydrated Au- mass-selected in the gas phase was studied. Probably the pump-photon can induce injection of an electron from auride chromophore to the H2O solvent. The cluster with 3 H2O mols. (Au-(H2O)3) showed a long-living excited state with a lifetime of ∼19 ± 3 ps, whereas that of Au-(H2O)2 is only ∼3 ± 1 ps. The fate of an optically excited state of an ionic species can be significantly changed by the no. of H2O (solvent) mols. attached. | eng |
| dc.description.version | published | |
| dc.identifier.citation | Chemical Physics Letters ; 588 (2013). - S. 27-30 | deu |
| dc.identifier.doi | 10.1016/j.cplett.2013.09.064 | deu |
| dc.identifier.ppn | 411071602 | deu |
| dc.identifier.uri | http://kops.uni-konstanz.de/handle/123456789/26614 | |
| dc.language.iso | eng | deu |
| dc.legacy.dateIssued | 2014-03-04 | deu |
| dc.rights | terms-of-use | deu |
| dc.rights.uri | https://rightsstatements.org/page/InC/1.0/ | deu |
| dc.subject | pump-probe spectroscopy | deu |
| dc.subject | solvation | deu |
| dc.subject | gold | deu |
| dc.subject.ddc | 540 | deu |
| dc.title | Relaxation dynamics of the mass-selected hydrated auride ion (Au<sup>-</sup>) | eng |
| dc.type | JOURNAL_ARTICLE | deu |
| dspace.entity.type | Publication | |
| kops.citation.bibtex | @article{Braun2013Relax-26614,
year={2013},
doi={10.1016/j.cplett.2013.09.064},
title={Relaxation dynamics of the mass-selected hydrated auride ion (Au<sup>-</sup>)},
volume={588},
issn={0009-2614},
journal={Chemical Physics Letters},
pages={27--30},
author={Braun, Christian and Pietsch, Susanne and Proch, Sebastian and Kim, Young Dok and Ganteför, Gerd},
note={Erratum to ‘Relaxation dynamics... ': We included above the corrected author list. One of the co-authors, Susanne Pietsch, was missing in the originally published Letter. The main contributions from Susanne Pietsch were the photoelectron spectra of Au−(H2O)m with m = 0–6 shown in Figure 1 measured with a photon energy of 7.9 eV. These data were critical to understand the data of the femtosecond time-resolved photoelectron spectroscopy. [Chemical Physics Letters ; https://doi.org/10.1016/j.cplett.2014.01.032]}
} | |
| kops.citation.iso690 | BRAUN, Christian, Susanne PIETSCH, Sebastian PROCH, Young Dok KIM, Gerd GANTEFÖR, 2013. Relaxation dynamics of the mass-selected hydrated auride ion (Au-). In: Chemical Physics Letters. 2013, 588, pp. 27-30. ISSN 0009-2614. eISSN 1873-4448. Available under: doi: 10.1016/j.cplett.2013.09.064 | deu |
| kops.citation.iso690 | BRAUN, Christian, Susanne PIETSCH, Sebastian PROCH, Young Dok KIM, Gerd GANTEFÖR, 2013. Relaxation dynamics of the mass-selected hydrated auride ion (Au-). In: Chemical Physics Letters. 2013, 588, pp. 27-30. ISSN 0009-2614. eISSN 1873-4448. Available under: doi: 10.1016/j.cplett.2013.09.064 | eng |
| kops.citation.rdf | <rdf:RDF
xmlns:dcterms="http://purl.org/dc/terms/"
xmlns:dc="http://purl.org/dc/elements/1.1/"
xmlns:rdf="http://www.w3.org/1999/02/22-rdf-syntax-ns#"
xmlns:bibo="http://purl.org/ontology/bibo/"
xmlns:dspace="http://digital-repositories.org/ontologies/dspace/0.1.0#"
xmlns:foaf="http://xmlns.com/foaf/0.1/"
xmlns:void="http://rdfs.org/ns/void#"
xmlns:xsd="http://www.w3.org/2001/XMLSchema#" >
<rdf:Description rdf:about="https://kops.uni-konstanz.de/server/rdf/resource/123456789/26614">
<dcterms:title>Relaxation dynamics of the mass-selected hydrated auride ion (Au<sup>-</sup>)</dcterms:title>
<dcterms:rights rdf:resource="https://rightsstatements.org/page/InC/1.0/"/>
<dc:creator>Kim, Young Dok</dc:creator>
<dc:rights>terms-of-use</dc:rights>
<dcterms:isPartOf rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/>
<dc:creator>Proch, Sebastian</dc:creator>
<dc:contributor>Kim, Young Dok</dc:contributor>
<dc:contributor>Ganteför, Gerd</dc:contributor>
<dspace:hasBitstream rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/26614/2/Braun_266146.pdf"/>
<dc:contributor>Proch, Sebastian</dc:contributor>
<dc:language>eng</dc:language>
<dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2014-03-04T09:56:33Z</dc:date>
<dc:creator>Pietsch, Susanne</dc:creator>
<dcterms:available rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2014-03-04T09:56:33Z</dcterms:available>
<dcterms:bibliographicCitation>Chemical Physics Letters ; 588 (2013). - S. 27-30</dcterms:bibliographicCitation>
<dc:creator>Braun, Christian</dc:creator>
<dcterms:hasPart rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/26614/2/Braun_266146.pdf"/>
<dcterms:issued>2013</dcterms:issued>
<void:sparqlEndpoint rdf:resource="http://localhost/fuseki/dspace/sparql"/>
<dspace:isPartOfCollection rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/>
<bibo:uri rdf:resource="http://kops.uni-konstanz.de/handle/123456789/26614"/>
<dc:contributor>Pietsch, Susanne</dc:contributor>
<dcterms:abstract xml:lang="eng">By using time-resolved photoelectron spectroscopy, decay of optically excited states of hydrated Au- mass-selected in the gas phase was studied. Probably the pump-photon can induce injection of an electron from auride chromophore to the H2O solvent. The cluster with 3 H2O mols. (Au-(H2O)3) showed a long-living excited state with a lifetime of ∼19 ± 3 ps, whereas that of Au-(H2O)2 is only ∼3 ± 1 ps. The fate of an optically excited state of an ionic species can be significantly changed by the no. of H2O (solvent) mols. attached.</dcterms:abstract>
<dc:creator>Ganteför, Gerd</dc:creator>
<dc:contributor>Braun, Christian</dc:contributor>
<foaf:homepage rdf:resource="http://localhost:8080/"/>
</rdf:Description>
</rdf:RDF> | |
| kops.description.comment | Erratum to ‘Relaxation dynamics... ': We included above the corrected author list. One of the co-authors, Susanne Pietsch, was missing in the originally published Letter. The main contributions from Susanne Pietsch were the photoelectron spectra of Au−(H2O)m with m = 0–6 shown in Figure 1 measured with a photon energy of 7.9 eV. These data were critical to understand the data of the femtosecond time-resolved photoelectron spectroscopy. [Chemical Physics Letters ; https://doi.org/10.1016/j.cplett.2014.01.032] | deu |
| kops.description.openAccess | openaccessgreen | |
| kops.flag.knbibliography | true | |
| kops.identifier.nbn | urn:nbn:de:bsz:352-266146 | deu |
| kops.sourcefield | Chemical Physics Letters. 2013, <b>588</b>, pp. 27-30. ISSN 0009-2614. eISSN 1873-4448. Available under: doi: 10.1016/j.cplett.2013.09.064 | deu |
| kops.sourcefield.plain | Chemical Physics Letters. 2013, 588, pp. 27-30. ISSN 0009-2614. eISSN 1873-4448. Available under: doi: 10.1016/j.cplett.2013.09.064 | deu |
| kops.sourcefield.plain | Chemical Physics Letters. 2013, 588, pp. 27-30. ISSN 0009-2614. eISSN 1873-4448. Available under: doi: 10.1016/j.cplett.2013.09.064 | eng |
| kops.submitter.email | sebastian.proch@uni-konstanz.de | deu |
| relation.isAuthorOfPublication | f217b1ab-7239-4c34-84b4-14287c922ba8 | |
| relation.isAuthorOfPublication | aa9f830e-3c67-4e5c-bb9a-5bf467c6e2a6 | |
| relation.isAuthorOfPublication | f0bc7b58-7a92-456e-80e9-a2d915c19db9 | |
| relation.isAuthorOfPublication | d81f0b28-9ec2-4bdb-b325-21714f128d3c | |
| relation.isAuthorOfPublication.latestForDiscovery | f217b1ab-7239-4c34-84b4-14287c922ba8 | |
| source.bibliographicInfo.fromPage | 27 | |
| source.bibliographicInfo.toPage | 30 | |
| source.bibliographicInfo.volume | 588 | |
| source.identifier.eissn | 1873-4448 | deu |
| source.identifier.issn | 0009-2614 | |
| source.periodicalTitle | Chemical Physics Letters |
Dateien
Originalbündel
1 - 1 von 1
Vorschaubild nicht verfügbar
- Name:
- Braun_266146.pdf
- Größe:
- 595.05 KB
- Format:
- Adobe Portable Document Format
Lizenzbündel
1 - 1 von 1
Vorschaubild nicht verfügbar
- Name:
- license.txt
- Größe:
- 1.92 KB
- Format:
- Plain Text
- Beschreibung:

