Spin torque–driven electron paramagnetic resonance of a single spin in a pentacene molecule

dc.contributor.authorKovarik, Stepan
dc.contributor.authorSchlitz, Richard
dc.contributor.authorVishwakarma, Aishwarya
dc.contributor.authorRuckert, Dominic
dc.contributor.authorGambardella, Pietro
dc.contributor.authorStepanow, Sebastian
dc.date.accessioned2024-12-06T12:06:27Z
dc.date.available2024-12-06T12:06:27Z
dc.date.issued2024-06-21
dc.description.abstractControl over quantum systems is typically achieved by time-dependent electric or magnetic fields. Alternatively, electronic spins can be controlled by spin-polarized currents. Here, we demonstrate coherent driving of a single spin by a radiofrequency spin-polarized current injected from the tip of a scanning tunneling microscope into an organic molecule. With the excitation of electron paramagnetic resonance, we established dynamic control of single spins by spin torque using a local electric current. In addition, our work highlights the dissipative action of the spin-transfer torque, in contrast to the nondissipative action of the magnetic field, which allows for the manipulation of individual spins based on controlled decoherence.
dc.description.versionpublisheddeu
dc.identifier.doi10.1126/science.adh4753
dc.identifier.urihttps://kops.uni-konstanz.de/handle/123456789/71597
dc.language.isoeng
dc.subject.ddc530
dc.titleSpin torque–driven electron paramagnetic resonance of a single spin in a pentacene moleculeeng
dc.typeJOURNAL_ARTICLE
dspace.entity.typePublication
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@article{Kovarik2024-06-21torqu-71597,
  year={2024},
  doi={10.1126/science.adh4753},
  title={Spin torque–driven electron paramagnetic resonance of a single spin in a pentacene molecule},
  number={6702},
  volume={384},
  issn={0036-8075},
  journal={Science},
  pages={1368--1373},
  author={Kovarik, Stepan and Schlitz, Richard and Vishwakarma, Aishwarya and Ruckert, Dominic and Gambardella, Pietro and Stepanow, Sebastian}
}
kops.citation.iso690KOVARIK, Stepan, Richard SCHLITZ, Aishwarya VISHWAKARMA, Dominic RUCKERT, Pietro GAMBARDELLA, Sebastian STEPANOW, 2024. Spin torque–driven electron paramagnetic resonance of a single spin in a pentacene molecule. In: Science. American Association for the Advancement of Science (AAAS). 2024, 384(6702), S. 1368-1373. ISSN 0036-8075. eISSN 1095-9203. Verfügbar unter: doi: 10.1126/science.adh4753deu
kops.citation.iso690KOVARIK, Stepan, Richard SCHLITZ, Aishwarya VISHWAKARMA, Dominic RUCKERT, Pietro GAMBARDELLA, Sebastian STEPANOW, 2024. Spin torque–driven electron paramagnetic resonance of a single spin in a pentacene molecule. In: Science. American Association for the Advancement of Science (AAAS). 2024, 384(6702), pp. 1368-1373. ISSN 0036-8075. eISSN 1095-9203. Available under: doi: 10.1126/science.adh4753eng
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