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Anisotropic magnetic properties of CeAg2Ge2 single crystals

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2006

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Thamizhavel, A.
Kulkarni, R.
Dhar, S. K.

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In order to investigate the anisotropic magnetic properties of CeAg2Ge2, we have successfully grown the single crystals, for the first time, by high temperature solution growth (flux) method. We have performed a detailed study of the grown single crystals by measuring their electrical resistivity, magnetic susceptibility, magnetization, specific heat and magnetoresistance. A clear anisotropy and an antiferromagnetic transition at TN = 4.6 K have been observed in the magnetic properties. The magnetic entropy reaches R ln 4 at 20 K indicating that the ground state and the first excited state are very closely spaced (a quasi-quartet state). From the specific heat measurements and crystalline electric field (CEF) analysis of the magnetic susceptibility, we have found the level splitting energies as 5 K and 130 K. The magnetization measurements reveal that the a-axis is the easy axis of magnetization and the saturation moment is μs = 1.6 μB/Ce, corroborating the previous neutron
scattering measurements on a polycrystalline sample.

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ISO 690THAMIZHAVEL, A., R. KULKARNI, S. K. DHAR, 2006. Anisotropic magnetic properties of CeAg2Ge2 single crystals
BibTex
@unpublished{Thamizhavel2006Aniso-9530,
  year={2006},
  doi={10.1103/PhysRevB.75.144426},
  title={Anisotropic magnetic properties of CeAg2Ge2 single crystals},
  author={Thamizhavel, A. and Kulkarni, R. and Dhar, S. K.}
}
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    <dcterms:abstract xml:lang="eng">In order to investigate the anisotropic magnetic properties of CeAg2Ge2, we have successfully grown the single crystals, for the first time, by high temperature solution growth (flux) method. We have performed a detailed study of the grown single crystals by measuring their electrical resistivity, magnetic susceptibility, magnetization, specific heat and magnetoresistance. A clear anisotropy and an antiferromagnetic transition at TN = 4.6 K have been observed in the magnetic properties. The magnetic entropy reaches R ln 4 at 20 K indicating that the ground state and the first excited state are very closely spaced (a quasi-quartet state). From the specific heat measurements and crystalline electric field (CEF) analysis of the magnetic susceptibility, we have found the level splitting energies as 5 K and 130 K. The magnetization measurements reveal that the a-axis is the easy axis of magnetization and the saturation moment is μs = 1.6 μB/Ce, corroborating the previous neutron&lt;br /&gt;scattering measurements on a polycrystalline sample.</dcterms:abstract>
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