Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters
| Type of Publication: | Journal article |
| URI (citable link): | http://nbn-resolving.de/urn:nbn:de:bsz:352-opus-85844 |
| Author: | Senz, Volkmar; Fischer, Tim; Oelßner, Patrice; Tiggesbäumker, Josef; Stanzel, Jörg; Bostedt, Christoph; Thomas, Heiko; Schöffler, Markus; Foucar, Lutz; Martins, Michael; Neville, John J.; Neeb, Matthias; Möller, Thomas; Wurth, Wilfried; Rühl, Eckart; Dörner, Reinhard; Schmidt-Böcking, Horst; Eberhardt, Wolfgang; Ganteför, Gerd; Treusch, Rolf; Radcliffe, Paul; Meiwes-Broer, Karl-Heinz |
| Year of publication: | 2009 |
| Published in: | Physical Review Letters ; 102 (2009). - 138303 |
| DOI (citable link): | https://dx.doi.org/10.1103/PhysRevLett.102.138303 |
| Summary: |
Metal clusters serve as model systems to study basic problems of electronic correlation. Vacuum ultraviolet light from the free-electron laser FLASH ionizes 5d electrons from mass-separated negatively charged clusters, thus transiently leading to core-ionized neutral systems. Shielding of the core hole affects the electron binding energy. From the strong deviation from expectations of the metallic droplet and jellium models we conclude on reduced electronic shielding once the cluster size falls below about 20 atoms. This suggests a metal-to-nonmetal transition, in agreement with previous local density approximation calculations.
|
| PACS Classification: | 73.22.-f; 41.60.Cr; 36.20.Kd; 36.40.Ei |
| Subject (DDC): | 530 Physics |
| Link to License: | In Copyright |
| Bibliography of Konstanz: | Yes |
Cite This
Files in this item
![[PDF]](/themes/Kops/images/mimes/pdf.png "PDF file"){kind=small}
SENZ, Volkmar, Tim FISCHER, Patrice OELSSNER, Josef TIGGESBÄUMKER, Jörg STANZEL, Christoph BOSTEDT, Heiko THOMAS, Markus SCHÖFFLER, Lutz FOUCAR, Michael MARTINS, John J. NEVILLE, Matthias NEEB, Thomas MÖLLER, Wilfried WURTH, Eckart RÜHL, Reinhard DÖRNER, Horst SCHMIDT-BÖCKING, Wolfgang EBERHARDT, Gerd GANTEFÖR, Rolf TREUSCH, Paul RADCLIFFE, Karl-Heinz MEIWES-BROER, 2009. Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters. In: Physical Review Letters. 102, 138303. Available under: doi: 10.1103/PhysRevLett.102.138303
@article{Senz2009CoreH-9113, title={Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters}, year={2009}, doi={10.1103/PhysRevLett.102.138303}, volume={102}, journal={Physical Review Letters}, author={Senz, Volkmar and Fischer, Tim and Oelßner, Patrice and Tiggesbäumker, Josef and Stanzel, Jörg and Bostedt, Christoph and Thomas, Heiko and Schöffler, Markus and Foucar, Lutz and Martins, Michael and Neville, John J. and Neeb, Matthias and Möller, Thomas and Wurth, Wilfried and Rühl, Eckart and Dörner, Reinhard and Schmidt-Böcking, Horst and Eberhardt, Wolfgang and Ganteför, Gerd and Treusch, Rolf and Radcliffe, Paul and Meiwes-Broer, Karl-Heinz}, note={Article Number: 138303} }
<rdf:RDF xmlns:dcterms="http://purl.org/dc/terms/" xmlns:dc="http://purl.org/dc/elements/1.1/" xmlns:rdf="http://www.w3.org/1999/02/22-rdf-syntax-ns#" xmlns:bibo="http://purl.org/ontology/bibo/" xmlns:dspace="http://digital-repositories.org/ontologies/dspace/0.1.0#" xmlns:foaf="http://xmlns.com/foaf/0.1/" xmlns:void="http://rdfs.org/ns/void#" xmlns:xsd="http://www.w3.org/2001/XMLSchema#" > <rdf:Description rdf:about="https://kops.uni-konstanz.de/rdf/resource/123456789/9113"> <dc:contributor>Schöffler, Markus</dc:contributor> <dc:format>application/pdf</dc:format> <dc:contributor>Ganteför, Gerd</dc:contributor> <dc:creator>Bostedt, Christoph</dc:creator> <dcterms:isPartOf rdf:resource="https://kops.uni-konstanz.de/rdf/resource/123456789/41"/> <dc:contributor>Foucar, Lutz</dc:contributor> <dc:creator>Neeb, Matthias</dc:creator> <void:sparqlEndpoint rdf:resource="http://localhost/fuseki/dspace/sparql"/> <dc:contributor>Radcliffe, Paul</dc:contributor> <dc:creator>Möller, Thomas</dc:creator> <dcterms:available rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2011-03-24T17:53:43Z</dcterms:available> <dc:language>eng</dc:language> <dc:contributor>Rühl, Eckart</dc:contributor> <dc:creator>Dörner, Reinhard</dc:creator> <dc:creator>Stanzel, Jörg</dc:creator> <dc:creator>Tiggesbäumker, Josef</dc:creator> <dc:creator>Oelßner, Patrice</dc:creator> <dc:creator>Meiwes-Broer, Karl-Heinz</dc:creator> <dc:contributor>Stanzel, Jörg</dc:contributor> <dc:contributor>Treusch, Rolf</dc:contributor> <dcterms:bibliographicCitation>First publ.in: Physical Review Letters 102 (2009), 138303</dcterms:bibliographicCitation> <dc:contributor>Tiggesbäumker, Josef</dc:contributor> <dc:creator>Foucar, Lutz</dc:creator> <dc:contributor>Schmidt-Böcking, Horst</dc:contributor> <dc:creator>Wurth, Wilfried</dc:creator> <dc:contributor>Senz, Volkmar</dc:contributor> <dc:contributor>Eberhardt, Wolfgang</dc:contributor> <dspace:isPartOfCollection rdf:resource="https://kops.uni-konstanz.de/rdf/resource/123456789/41"/> <dcterms:title>Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters</dcterms:title> <dc:rights>terms-of-use</dc:rights> <dc:contributor>Wurth, Wilfried</dc:contributor> <dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2011-03-24T17:53:43Z</dc:date> <dc:contributor>Neville, John J.</dc:contributor> <dc:creator>Rühl, Eckart</dc:creator> <dc:creator>Ganteför, Gerd</dc:creator> <dc:contributor>Dörner, Reinhard</dc:contributor> <dspace:hasBitstream rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/9113/1/PhysRevLett102.pdf"/> <dcterms:rights rdf:resource="https://rightsstatements.org/page/InC/1.0/"/> <dcterms:hasPart rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/9113/1/PhysRevLett102.pdf"/> <dc:creator>Martins, Michael</dc:creator> <dc:contributor>Oelßner, Patrice</dc:contributor> <dc:contributor>Martins, Michael</dc:contributor> <dc:contributor>Thomas, Heiko</dc:contributor> <bibo:uri rdf:resource="http://kops.uni-konstanz.de/handle/123456789/9113"/> <dc:creator>Thomas, Heiko</dc:creator> <foaf:homepage rdf:resource="http://localhost:8080/jspui"/> <dc:creator>Radcliffe, Paul</dc:creator> <dc:contributor>Meiwes-Broer, Karl-Heinz</dc:contributor> <dc:creator>Eberhardt, Wolfgang</dc:creator> <dc:creator>Senz, Volkmar</dc:creator> <dc:contributor>Fischer, Tim</dc:contributor> <dc:creator>Schöffler, Markus</dc:creator> <dc:contributor>Bostedt, Christoph</dc:contributor> <dc:creator>Treusch, Rolf</dc:creator> <dc:contributor>Möller, Thomas</dc:contributor> <dc:creator>Schmidt-Böcking, Horst</dc:creator> <dc:creator>Fischer, Tim</dc:creator> <dc:creator>Neville, John J.</dc:creator> <dcterms:issued>2009</dcterms:issued> <dcterms:abstract xml:lang="eng">Metal clusters serve as model systems to study basic problems of electronic correlation. Vacuum ultraviolet light from the free-electron laser FLASH ionizes 5d electrons from mass-separated negatively charged clusters, thus transiently leading to core-ionized neutral systems. Shielding of the core hole affects the electron binding energy. From the strong deviation from expectations of the metallic droplet and jellium models we conclude on reduced electronic shielding once the cluster size falls below about 20 atoms. This suggests a metal-to-nonmetal transition, in agreement with previous local density approximation calculations.</dcterms:abstract> <dc:contributor>Neeb, Matthias</dc:contributor> </rdf:Description> </rdf:RDF>
Downloads since Oct 1, 2014 (Information about access statistics)
| PhysRevLett102.pdf | 258 |
This item appears in the following Collection(s)
Search KOPS
Browse
My Account
