Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters
Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters
Date
2009
Authors
Senz, Volkmar
Oelßner, Patrice
Tiggesbäumker, Josef
Stanzel, Jörg
Bostedt, Christoph
Thomas, Heiko
Schöffler, Markus
Foucar, Lutz
Martins, Michael
Editors
Journal ISSN
Electronic ISSN
ISBN
Bibliographical data
Publisher
Series
URI (citable link)
DOI (citable link)
International patent number
Link to the license
EU project number
Project
Open Access publication
Collections
Title in another language
Publication type
Journal article
Publication status
Published in
Physical Review Letters ; 102 (2009). - 138303
Abstract
Metal clusters serve as model systems to study basic problems of electronic correlation. Vacuum ultraviolet light from the free-electron laser FLASH ionizes 5d electrons from mass-separated negatively charged clusters, thus transiently leading to core-ionized neutral systems. Shielding of the core hole affects the electron binding energy. From the strong deviation from expectations of the metallic droplet and jellium models we conclude on reduced electronic shielding once the cluster size falls below about 20 atoms. This suggests a metal-to-nonmetal transition, in agreement with previous local density approximation calculations.
Summary in another language
Subject (DDC)
530 Physics
Keywords
Conference
Review
undefined / . - undefined, undefined. - (undefined; undefined)
Cite This
ISO 690
SENZ, Volkmar, Tim FISCHER, Patrice OELSSNER, Josef TIGGESBÄUMKER, Jörg STANZEL, Christoph BOSTEDT, Heiko THOMAS, Markus SCHÖFFLER, Lutz FOUCAR, Michael MARTINS, John J. NEVILLE, Matthias NEEB, Thomas MÖLLER, Wilfried WURTH, Eckart RÜHL, Reinhard DÖRNER, Horst SCHMIDT-BÖCKING, Wolfgang EBERHARDT, Gerd GANTEFÖR, Rolf TREUSCH, Paul RADCLIFFE, Karl-Heinz MEIWES-BROER, 2009. Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters. In: Physical Review Letters. 102, 138303. Available under: doi: 10.1103/PhysRevLett.102.138303BibTex
@article{Senz2009CoreH-9113, year={2009}, doi={10.1103/PhysRevLett.102.138303}, title={Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters}, volume={102}, journal={Physical Review Letters}, author={Senz, Volkmar and Fischer, Tim and Oelßner, Patrice and Tiggesbäumker, Josef and Stanzel, Jörg and Bostedt, Christoph and Thomas, Heiko and Schöffler, Markus and Foucar, Lutz and Martins, Michael and Neville, John J. and Neeb, Matthias and Möller, Thomas and Wurth, Wilfried and Rühl, Eckart and Dörner, Reinhard and Schmidt-Böcking, Horst and Eberhardt, Wolfgang and Ganteför, Gerd and Treusch, Rolf and Radcliffe, Paul and Meiwes-Broer, Karl-Heinz}, note={Article Number: 138303} }
RDF
<rdf:RDF xmlns:dcterms="http://purl.org/dc/terms/" xmlns:dc="http://purl.org/dc/elements/1.1/" xmlns:rdf="http://www.w3.org/1999/02/22-rdf-syntax-ns#" xmlns:bibo="http://purl.org/ontology/bibo/" xmlns:dspace="http://digital-repositories.org/ontologies/dspace/0.1.0#" xmlns:foaf="http://xmlns.com/foaf/0.1/" xmlns:void="http://rdfs.org/ns/void#" xmlns:xsd="http://www.w3.org/2001/XMLSchema#" > <rdf:Description rdf:about="https://kops.uni-konstanz.de/server/rdf/resource/123456789/9113"> <dc:creator>Neeb, Matthias</dc:creator> <dspace:hasBitstream rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/9113/1/PhysRevLett102.pdf"/> <dc:contributor>Ganteför, Gerd</dc:contributor> <dcterms:abstract xml:lang="eng">Metal clusters serve as model systems to study basic problems of electronic correlation. Vacuum ultraviolet light from the free-electron laser FLASH ionizes 5d electrons from mass-separated negatively charged clusters, thus transiently leading to core-ionized neutral systems. Shielding of the core hole affects the electron binding energy. From the strong deviation from expectations of the metallic droplet and jellium models we conclude on reduced electronic shielding once the cluster size falls below about 20 atoms. This suggests a metal-to-nonmetal transition, in agreement with previous local density approximation calculations.</dcterms:abstract> <dc:creator>Eberhardt, Wolfgang</dc:creator> <dc:contributor>Dörner, Reinhard</dc:contributor> <dc:creator>Oelßner, Patrice</dc:creator> <dc:contributor>Rühl, Eckart</dc:contributor> <dcterms:bibliographicCitation>First publ.in: Physical Review Letters 102 (2009), 138303</dcterms:bibliographicCitation> <dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2011-03-24T17:53:43Z</dc:date> <dc:creator>Martins, Michael</dc:creator> <foaf:homepage rdf:resource="http://localhost:8080/"/> <dc:creator>Radcliffe, Paul</dc:creator> <dspace:isPartOfCollection rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/> <dc:contributor>Neeb, Matthias</dc:contributor> <dc:creator>Wurth, Wilfried</dc:creator> <dc:contributor>Oelßner, Patrice</dc:contributor> <dc:creator>Schmidt-Böcking, Horst</dc:creator> <dc:creator>Ganteför, Gerd</dc:creator> <dc:contributor>Radcliffe, Paul</dc:contributor> <dc:creator>Dörner, Reinhard</dc:creator> <dc:contributor>Wurth, Wilfried</dc:contributor> <dc:contributor>Stanzel, Jörg</dc:contributor> <dc:contributor>Meiwes-Broer, Karl-Heinz</dc:contributor> <dcterms:isPartOf rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/> <dc:contributor>Fischer, Tim</dc:contributor> <dcterms:issued>2009</dcterms:issued> <dc:contributor>Eberhardt, Wolfgang</dc:contributor> <dc:contributor>Foucar, Lutz</dc:contributor> <dc:creator>Möller, Thomas</dc:creator> <void:sparqlEndpoint rdf:resource="http://localhost/fuseki/dspace/sparql"/> <dc:contributor>Bostedt, Christoph</dc:contributor> <dc:creator>Fischer, Tim</dc:creator> <dc:contributor>Neville, John J.</dc:contributor> <dc:format>application/pdf</dc:format> <bibo:uri rdf:resource="http://kops.uni-konstanz.de/handle/123456789/9113"/> <dc:creator>Bostedt, Christoph</dc:creator> <dc:creator>Thomas, Heiko</dc:creator> <dcterms:rights rdf:resource="https://rightsstatements.org/page/InC/1.0/"/> <dc:contributor>Thomas, Heiko</dc:contributor> <dc:contributor>Treusch, Rolf</dc:contributor> <dc:creator>Stanzel, Jörg</dc:creator> <dc:creator>Foucar, Lutz</dc:creator> <dc:creator>Treusch, Rolf</dc:creator> <dc:contributor>Schmidt-Böcking, Horst</dc:contributor> <dc:creator>Meiwes-Broer, Karl-Heinz</dc:creator> <dc:contributor>Martins, Michael</dc:contributor> <dc:contributor>Senz, Volkmar</dc:contributor> <dc:creator>Rühl, Eckart</dc:creator> <dc:creator>Schöffler, Markus</dc:creator> <dc:creator>Senz, Volkmar</dc:creator> <dc:language>eng</dc:language> <dcterms:title>Core-Hole Screening as a Probe for a Metal-to-Nonmetal Transition in Lead Clusters</dcterms:title> <dc:contributor>Schöffler, Markus</dc:contributor> <dc:contributor>Möller, Thomas</dc:contributor> <dc:rights>terms-of-use</dc:rights> <dc:contributor>Tiggesbäumker, Josef</dc:contributor> <dc:creator>Tiggesbäumker, Josef</dc:creator> <dc:creator>Neville, John J.</dc:creator> <dcterms:available rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2011-03-24T17:53:43Z</dcterms:available> <dcterms:hasPart rdf:resource="https://kops.uni-konstanz.de/bitstream/123456789/9113/1/PhysRevLett102.pdf"/> </rdf:Description> </rdf:RDF>
Internal note
xmlui.Submission.submit.DescribeStep.inputForms.label.kops_note_fromSubmitter
Examination date of dissertation
Method of financing
Comment on publication
Alliance license
Corresponding Authors der Uni Konstanz vorhanden
International Co-Authors
Bibliography of Konstanz
Yes