Femtosecond phononic coupling to both spins and charges in a room temperature antiferromagnetic semiconductor
Femtosecond phononic coupling to both spins and charges in a room temperature antiferromagnetic semiconductor
No Thumbnail Available
Files
There are no files associated with this item.
Date
2021
Authors
Dal Conte, Stefano
Terschanski, Marc
Springholz, Gunther
Bonanni, Alberta
Deltenre, Kira
Anders, Frithjof B.
Uhrig, Götz S.
Cerullo, Giulio
Cinchetti, Mirko
Editors
Journal ISSN
Electronic ISSN
ISBN
Bibliographical data
Publisher
Series
DOI (citable link)
ArXiv-ID
International patent number
Link to the license
oops
EU project number
Project
Open Access publication
Collections
Title in another language
Publication type
Journal article
Publication status
Published
Published in
Physical Review B ; 104 (2021), 22. - 224424. - American Physical Society (APS). - ISSN 2469-9950. - eISSN 2469-9969
Abstract
Spintronics is postulated on the possibility to employ the magnetic degree of freedom of electrons for computation and couple it to charges. In this view the combination of the high frequency of spin manipulations offered by antiferromagnets, with the wide tunability of the electronic properties peculiar of semiconductors, provides a promising and intriguing platform. Here we explore this scenario in α-MnTe, which is a semiconductor antiferromagnetically ordered at room temperature. Relying on a Raman mechanism and femtosecond laser pulses, we drive degenerate modes of coherent optical phonons, which modulate the chemical bonds involved in the superexchange interaction. The spectrally resolved measurements of the transient reflectivity reveal a coherent modulation of the band gap at the frequency of 5.3 THz. The detection of the rotation of the polarization, typically associated with magneto-optical effects, shows coherent and incoherent contributions. Modeling how the ionic motion induced by the phonons affects the exchange interaction in the material, we calculate the photoinduced THz spin dynamics: the results predict both a coherent and incoherent response, the latter of which is consistent with the experimental observation. Our work demonstrates that the same phonon modes modulate both the charge and magnetic degree of freedom, suggesting the resonant pumping of phonons as a viable way to link spin and charge dynamics even in nonlinear regimes.
Summary in another language
Subject (DDC)
530 Physics
Keywords
Conference
Review
undefined / . - undefined, undefined. - (undefined; undefined)
Cite This
ISO 690
BOSSINI, Davide, Stefano DAL CONTE, Marc TERSCHANSKI, Gunther SPRINGHOLZ, Alberta BONANNI, Kira DELTENRE, Frithjof B. ANDERS, Götz S. UHRIG, Giulio CERULLO, Mirko CINCHETTI, 2021. Femtosecond phononic coupling to both spins and charges in a room temperature antiferromagnetic semiconductor. In: Physical Review B. American Physical Society (APS). 104(22), 224424. ISSN 2469-9950. eISSN 2469-9969. Available under: doi: 10.1103/PhysRevB.104.224424BibTex
@article{Bossini2021-10-28T14:50:15ZFemto-56073, year={2021}, doi={10.1103/PhysRevB.104.224424}, title={Femtosecond phononic coupling to both spins and charges in a room temperature antiferromagnetic semiconductor}, number={22}, volume={104}, issn={2469-9950}, journal={Physical Review B}, author={Bossini, Davide and Dal Conte, Stefano and Terschanski, Marc and Springholz, Gunther and Bonanni, Alberta and Deltenre, Kira and Anders, Frithjof B. and Uhrig, Götz S. and Cerullo, Giulio and Cinchetti, Mirko}, note={Article Number: 224424} }
RDF
<rdf:RDF xmlns:dcterms="http://purl.org/dc/terms/" xmlns:dc="http://purl.org/dc/elements/1.1/" xmlns:rdf="http://www.w3.org/1999/02/22-rdf-syntax-ns#" xmlns:bibo="http://purl.org/ontology/bibo/" xmlns:dspace="http://digital-repositories.org/ontologies/dspace/0.1.0#" xmlns:foaf="http://xmlns.com/foaf/0.1/" xmlns:void="http://rdfs.org/ns/void#" xmlns:xsd="http://www.w3.org/2001/XMLSchema#" > <rdf:Description rdf:about="https://kops.uni-konstanz.de/server/rdf/resource/123456789/56073"> <void:sparqlEndpoint rdf:resource="http://localhost/fuseki/dspace/sparql"/> <dc:creator>Springholz, Gunther</dc:creator> <dc:contributor>Terschanski, Marc</dc:contributor> <dc:creator>Cinchetti, Mirko</dc:creator> <dc:creator>Bonanni, Alberta</dc:creator> <dc:contributor>Dal Conte, Stefano</dc:contributor> <dc:contributor>Cerullo, Giulio</dc:contributor> <dc:contributor>Anders, Frithjof B.</dc:contributor> <dc:contributor>Bossini, Davide</dc:contributor> <dc:contributor>Springholz, Gunther</dc:contributor> <dcterms:abstract xml:lang="eng">Spintronics is postulated on the possibility to employ the magnetic degree of freedom of electrons for computation and couple it to charges. In this view the combination of the high frequency of spin manipulations offered by antiferromagnets, with the wide tunability of the electronic properties peculiar of semiconductors, provides a promising and intriguing platform. Here we explore this scenario in α-MnTe, which is a semiconductor antiferromagnetically ordered at room temperature. Relying on a Raman mechanism and femtosecond laser pulses, we drive degenerate modes of coherent optical phonons, which modulate the chemical bonds involved in the superexchange interaction. The spectrally resolved measurements of the transient reflectivity reveal a coherent modulation of the band gap at the frequency of 5.3 THz. The detection of the rotation of the polarization, typically associated with magneto-optical effects, shows coherent and incoherent contributions. Modeling how the ionic motion induced by the phonons affects the exchange interaction in the material, we calculate the photoinduced THz spin dynamics: the results predict both a coherent and incoherent response, the latter of which is consistent with the experimental observation. Our work demonstrates that the same phonon modes modulate both the charge and magnetic degree of freedom, suggesting the resonant pumping of phonons as a viable way to link spin and charge dynamics even in nonlinear regimes.</dcterms:abstract> <foaf:homepage rdf:resource="http://localhost:8080/"/> <dcterms:title>Femtosecond phononic coupling to both spins and charges in a room temperature antiferromagnetic semiconductor</dcterms:title> <dc:contributor>Deltenre, Kira</dc:contributor> <dcterms:isPartOf rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/> <dcterms:available rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2022-01-05T08:01:38Z</dcterms:available> <dc:creator>Uhrig, Götz S.</dc:creator> <bibo:uri rdf:resource="https://kops.uni-konstanz.de/handle/123456789/56073"/> <dc:language>eng</dc:language> <dspace:isPartOfCollection rdf:resource="https://kops.uni-konstanz.de/server/rdf/resource/123456789/41"/> <dc:creator>Bossini, Davide</dc:creator> <dc:contributor>Uhrig, Götz S.</dc:contributor> <dc:contributor>Cinchetti, Mirko</dc:contributor> <dc:creator>Dal Conte, Stefano</dc:creator> <dc:creator>Deltenre, Kira</dc:creator> <dc:creator>Terschanski, Marc</dc:creator> <dc:creator>Anders, Frithjof B.</dc:creator> <dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2022-01-05T08:01:38Z</dc:date> <dc:contributor>Bonanni, Alberta</dc:contributor> <dcterms:issued>2021-10-28T14:50:15Z</dcterms:issued> <dc:creator>Cerullo, Giulio</dc:creator> </rdf:Description> </rdf:RDF>
Internal note
xmlui.Submission.submit.DescribeStep.inputForms.label.kops_note_fromSubmitter
Examination date of dissertation
Method of financing
Comment on publication
Alliance license
Corresponding Authors der Uni Konstanz vorhanden
International Co-Authors
Bibliography of Konstanz
Yes
Refereed
Yes