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One-dimensional (Mo3S3)n clusters : building blocks of clusters materials and ideal nanowires for molecular electronics

One-dimensional (Mo3S3)n clusters : building blocks of clusters materials and ideal nanowires for molecular electronics

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GEMMING, Sibylle, Gotthard SEIFERT, Nils BERTRAM, Tim FISCHER, Matthias GÖTZ, Gerd GANTEFÖR, 2009. One-dimensional (Mo3S3)n clusters : building blocks of clusters materials and ideal nanowires for molecular electronics. In: Chemical Physics Letters. 474(1-3), pp. 127-131

@article{Gemming2009One-d-5322, title={One-dimensional (Mo3S3)n clusters : building blocks of clusters materials and ideal nanowires for molecular electronics}, year={2009}, doi={10.1016/j.cplett.2009.04.020}, number={1-3}, volume={474}, journal={Chemical Physics Letters}, pages={127--131}, author={Gemming, Sibylle and Seifert, Gotthard and Bertram, Nils and Fischer, Tim and Götz, Matthias and Ganteför, Gerd} }

<rdf:RDF xmlns:rdf="http://www.w3.org/1999/02/22-rdf-syntax-ns#" xmlns:bibo="http://purl.org/ontology/bibo/" xmlns:dc="http://purl.org/dc/elements/1.1/" xmlns:dcterms="http://purl.org/dc/terms/" xmlns:xsd="http://www.w3.org/2001/XMLSchema#" > <rdf:Description rdf:about="https://kops.uni-konstanz.de/rdf/resource/123456789/5322"> <dcterms:abstract xml:lang="eng">The geometric and electronic structures of gas phase (Mo3S3)nS2 and (Mo3S3)n-1(MoS4)2 clusters with n = 2, 3, 4, . . . are studied experimentally using mass and photoelectron spectroscopy. The Mo3S3 units form one-dimensional chains with length n . There are two possible types of terminations at the ends: a single S atom or a MoS4 cluster. The experimental results are compared to calculations based on density- functional theory. Although clusters of this type have been known for decades as constituents of Chevrel phases, we here report their first gas phase synthesis for sizes up to n = 17. With increasing n, the gap vanishes extending such clusters to a conducting wire.</dcterms:abstract> <dc:creator>Ganteför, Gerd</dc:creator> <dc:creator>Götz, Matthias</dc:creator> <dc:rights>deposit-license</dc:rights> <dc:contributor>Seifert, Gotthard</dc:contributor> <dc:creator>Gemming, Sibylle</dc:creator> <dc:format>application/pdf</dc:format> <dcterms:issued>2009</dcterms:issued> <bibo:uri rdf:resource="http://kops.uni-konstanz.de/handle/123456789/5322"/> <dc:contributor>Ganteför, Gerd</dc:contributor> <dcterms:bibliographicCitation>First publ. in: Chemical Physics Letters 474 (2009), 1-3, pp. 127 131</dcterms:bibliographicCitation> <dc:creator>Fischer, Tim</dc:creator> <dc:contributor>Gemming, Sibylle</dc:contributor> <dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2011-03-24T14:54:55Z</dc:date> <dc:creator>Seifert, Gotthard</dc:creator> <dc:language>deu</dc:language> <dcterms:rights rdf:resource="http://nbn-resolving.org/urn:nbn:de:bsz:352-20140905103416863-3868037-7"/> <dcterms:title>One-dimensional (Mo3S3)n clusters : building blocks of clusters materials and ideal nanowires for molecular electronics</dcterms:title> <dc:contributor>Fischer, Tim</dc:contributor> <dc:contributor>Bertram, Nils</dc:contributor> <dcterms:available rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2011-03-24T14:54:55Z</dcterms:available> <dc:contributor>Götz, Matthias</dc:contributor> <dc:creator>Bertram, Nils</dc:creator> </rdf:Description> </rdf:RDF>

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