Theory of thermodynamic stresses in colloidal dispersions at the glass transition
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| Type of Publication: | Preprint |
| URI (citable link): | http://nbn-resolving.de/urn:nbn:de:bsz:352-opus-73949 |
| Author: | Hajnal, David; Henrich, Oliver; Crassous, Jérôme J.; Siebenbürger, Miriam; Drechsler, Markus; Ballauff, Matthias; Fuchs, Matthias |
| Year of publication: | 2008 |
| ArXiv-ID: | arXiv:0805.0652v1 |
| DOI (citable link): | https://dx.doi.org/10.1063/1.2964805 |
| Summary: |
We discuss the nonlinear rheology of dense colloidal dispersions at the glass transition. A first principles approach starting with interacting Brownian particles in given arbitrary homogeneous (incompressible) flow neglecting hydrodynamic interactions is sketched. It e.g. explains steady state flow curves for finite shear rates measured in dense suspensions of thermosensitive core-shell particles consisting of a polystyrene core and a crosslinked poly(N-isopropylacrylamide)(PNIPAM) shell. The exponents of simple and generalized Herschel Bulkley laws are computed for hard spheres.
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| PACS Classification: | 83.60.Fg; 82.70.Dd; 64.70.P-; 83.50.Ax; 83.60.Df |
| Subject (DDC): | 530 Physics |
| Link to License: | Attribution-NonCommercial-NoDerivs 2.0 Generic |
| Bibliography of Konstanz: | Yes |
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HAJNAL, David, Oliver HENRICH, Jérôme J. CRASSOUS, Miriam SIEBENBÜRGER, Markus DRECHSLER, Matthias BALLAUFF, Matthias FUCHS, 2008. Theory of thermodynamic stresses in colloidal dispersions at the glass transition. Available under: doi: 10.1063/1.2964805
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