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Polymer-Mode-Coupling Theory of Finite-Size-Fluctuation Effects in Entangled Solutions, Melts, and Gels. 1. General Formulation and Predictions

Polymer-Mode-Coupling Theory of Finite-Size-Fluctuation Effects in Entangled Solutions, Melts, and Gels. 1. General Formulation and Predictions

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FUCHS, Matthias, Kenneth S. SCHWEIZER, 1997. Polymer-Mode-Coupling Theory of Finite-Size-Fluctuation Effects in Entangled Solutions, Melts, and Gels. 1. General Formulation and Predictions. In: Macromolecules. 30, pp. 5133-5155

@article{Fuchs1997Polym-4936, title={Polymer-Mode-Coupling Theory of Finite-Size-Fluctuation Effects in Entangled Solutions, Melts, and Gels. 1. General Formulation and Predictions}, year={1997}, doi={10.1021/ma970234b}, volume={30}, journal={Macromolecules}, pages={5133--5155}, author={Fuchs, Matthias and Schweizer, Kenneth S.} }

<rdf:RDF xmlns:rdf="http://www.w3.org/1999/02/22-rdf-syntax-ns#" xmlns:bibo="http://purl.org/ontology/bibo/" xmlns:dc="http://purl.org/dc/elements/1.1/" xmlns:dcterms="http://purl.org/dc/terms/" xmlns:xsd="http://www.w3.org/2001/XMLSchema#" > <rdf:Description rdf:about="https://kops.uni-konstanz.de/rdf/resource/123456789/4936"> <dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2011-03-24T14:51:30Z</dc:date> <dcterms:rights rdf:resource="https://creativecommons.org/licenses/by-nc-nd/2.0/legalcode"/> <dcterms:available rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2011-03-24T14:51:30Z</dcterms:available> <dc:contributor>Fuchs, Matthias</dc:contributor> <dcterms:title>Polymer-Mode-Coupling Theory of Finite-Size-Fluctuation Effects in Entangled Solutions, Melts, and Gels. 1. General Formulation and Predictions</dcterms:title> <dcterms:abstract xml:lang="eng">The transport coefficients of dense polymeric fluids are approximately calculated from the microscopic intermolecular forces. The following finite molecular weight effects are discussed within the polymer-mode-coupling theory (PMC) and compared to the corresponding reptation/tube ideas: constraint release mechanism, spatial inhomogeneity of the entanglement constraints, and tracer polymer shape fluctuations. The entanglement corrections to the single polymer Rouse dynamics are shown to depend on molecular weight via the ratio N/Ne, where the entanglement degree of polymerization, Ne, can be measured from the plateau shear modulus.</dcterms:abstract> <dc:creator>Fuchs, Matthias</dc:creator> <dc:format>application/pdf</dc:format> <bibo:uri rdf:resource="http://kops.uni-konstanz.de/handle/123456789/4936"/> <dcterms:issued>1997</dcterms:issued> <dc:creator>Schweizer, Kenneth S.</dc:creator> <dcterms:bibliographicCitation>First publ. in: Macromolecules 30 (1997), pp. 5133-5155</dcterms:bibliographicCitation> <dc:rights>deposit-license</dc:rights> <dc:language>eng</dc:language> <dc:contributor>Schweizer, Kenneth S.</dc:contributor> </rdf:Description> </rdf:RDF>

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