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Type of Publication: | Journal article |
URI (citable link): | http://nbn-resolving.de/urn:nbn:de:bsz:352-opus-36704 |
Author: | Fuchs, Matthias; Götze, Wolfgang; Mayr, Matthias R. |
Year of publication: | 1998 |
Published in: | Physical Review E ; 58 (1998), 3. - pp. 3384-3399 |
DOI (citable link): | https://dx.doi.org/10.1103/PhysRevE.58.3384 |
Summary: |
Within mode-coupling theory for structural relaxation in simple systems, the asymptotic laws and their leading-asymptotic correction formulas are derived for the motion of a tagged particle near a glass-transition singularity. These analytic results are compared with numerical ones of the equations of motion evaluated for a tagged hard sphere moving in a hard-sphere system. It is found that the long-time part of the two-step relaxation process for the mean-squared displacement can be characterized by the a-relaxation scaling law and von Schweidlers power-law decay, while the critical-decay regime is dominated by the corrections to the leading power-law behavior. For parameters of interest for the interpretations of experimental data, the corrections to the leading asymptotic laws for the non-Gaussian parameter are found to be so large that the leading asymptotic results are altered qualitatively by the corrections. Results for the non-Gaussian parameter are shown to follow qualitatively the findings reported in the molecular-dynamics-simulations work by Kob and Andersen [Phys. Rev. E 51, 4626 (1995)].
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PACS Classification: | 64.70.Pf; 61.20.Lc |
Subject (DDC): | 530 Physics |
Link to License: | Attribution-NonCommercial-NoDerivs 2.0 Generic |
FUCHS, Matthias, Wolfgang GÖTZE, Matthias R. MAYR, 1998. Asymptotic laws for tagged-particle motion in glassy systems. In: Physical Review E. 58(3), pp. 3384-3399. Available under: doi: 10.1103/PhysRevE.58.3384
@article{Fuchs1998Asymp-4875, title={Asymptotic laws for tagged-particle motion in glassy systems}, year={1998}, doi={10.1103/PhysRevE.58.3384}, number={3}, volume={58}, journal={Physical Review E}, pages={3384--3399}, author={Fuchs, Matthias and Götze, Wolfgang and Mayr, Matthias R.} }
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