Shell structure and s-p hybridization in small aluminum clusters


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GANTEFÖR, Gerd, Wolfgang EBERHARDT, 1994. Shell structure and s-p hybridization in small aluminum clusters. In: Chemical Physics Letters. 217(5-6), pp. 600-604

@article{Gantefor1994Shell-4653, title={Shell structure and s-p hybridization in small aluminum clusters}, year={1994}, doi={10.1016/0009-2614(93)E1436-K}, number={5-6}, volume={217}, journal={Chemical Physics Letters}, pages={600--604}, author={Ganteför, Gerd and Eberhardt, Wolfgang} }

<rdf:RDF xmlns:rdf="" xmlns:bibo="" xmlns:dc="" xmlns:dcterms="" xmlns:xsd="" > <rdf:Description rdf:about=""> <dc:creator>Ganteför, Gerd</dc:creator> <dc:creator>Eberhardt, Wolfgang</dc:creator> <dc:date rdf:datatype="">2011-03-24T14:49:18Z</dc:date> <dcterms:issued>1994</dcterms:issued> <dc:language>eng</dc:language> <dcterms:available rdf:datatype="">2011-03-24T14:49:18Z</dcterms:available> <dc:rights>deposit-license</dc:rights> <dc:contributor>Ganteför, Gerd</dc:contributor> <dc:format>application/pdf</dc:format> <dcterms:title>Shell structure and s-p hybridization in small aluminum clusters</dcterms:title> <dc:contributor>Eberhardt, Wolfgang</dc:contributor> <dcterms:bibliographicCitation>First publ. in: Chemical Physics Letters 217 (1994), 5-6, pp. 600-604</dcterms:bibliographicCitation> <bibo:uri rdf:resource=""/> <dcterms:abstract xml:lang="eng">Photoelectron spectra of Al−n (n=2 20) clusters are presented. Due to the improved energy resolution and the relatively high photon energy (hv=6.424 eV, ArF laser radiation) available in our experiment the spectra reveal the mechanism of the onset of the s p hybridization occuring in these particles. Between Al−6 Al−12 a mixing of the uppermost antibonding 3s derived orbital with the 3p band takes place which is observed simultaneously with the 2D→3D structural transition predicted for Al clusters in this size range. Starting from Al−13 a pattern resembling an electronic shell structure is identified.</dcterms:abstract> <dcterms:rights rdf:resource=""/> </rdf:Description> </rdf:RDF>

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