Interactions and Magnetotransport through Spin-Valley Coupled Landau Levels in Monolayer MoS2

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2018
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Pisoni, Riccardo
Lei, Zijin
Back, Patrick
Eich, Marius
Overweg, Hiske
Lee, Yongjin
Rickhaus, Peter
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Physical Review Letters. 2018, 121(24), 247701. ISSN 0031-9007. eISSN 1079-7114. Available under: doi: 10.1103/PhysRevLett.121.247701
Zusammenfassung

The strong spin-orbit coupling and the broken inversion symmetry in monolayer transition metal dichalcogenides results in spin-valley coupled band structures. Such a band structure leads to novel applications in the fields of electronics and optoelectronics. Density functional theory calculations as well as optical experiments have focused on spin-valley coupling in the valence band. Here we present magnetotransport experiments on high-quality n-type monolayer molybdenum disulphide (MoS2) samples, displaying highly resolved Shubnikov–de Haas oscillations at magnetic fields as low as 2 T. We find the effective mass 0.7me, about twice as large as theoretically predicted and almost independent of magnetic field and carrier density. We further detect the occupation of the second spin-orbit split band at an energy of about 15 meV, i.e., about a factor of 5 larger than predicted. In addition, we demonstrate an intricate Landau level spectrum arising from a complex interplay between a density-dependent Zeeman splitting and spin- and valley-split Landau levels. These observations, enabled by the high electronic quality of our samples, testify to the importance of interaction effects in the conduction band of monolayer MoS2.

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ISO 690PISONI, Riccardo, Andor KORMÁNYOS, Matthew BROOKS, Zijin LEI, Patrick BACK, Marius EICH, Hiske OVERWEG, Yongjin LEE, Peter RICKHAUS, Guido BURKARD, 2018. Interactions and Magnetotransport through Spin-Valley Coupled Landau Levels in Monolayer MoS2. In: Physical Review Letters. 2018, 121(24), 247701. ISSN 0031-9007. eISSN 1079-7114. Available under: doi: 10.1103/PhysRevLett.121.247701
BibTex
@article{Pisoni2018Inter-45126,
  year={2018},
  doi={10.1103/PhysRevLett.121.247701},
  title={Interactions and Magnetotransport through Spin-Valley Coupled Landau Levels in Monolayer MoS<sub>2</sub>},
  number={24},
  volume={121},
  issn={0031-9007},
  journal={Physical Review Letters},
  author={Pisoni, Riccardo and Kormányos, Andor and Brooks, Matthew and Lei, Zijin and Back, Patrick and Eich, Marius and Overweg, Hiske and Lee, Yongjin and Rickhaus, Peter and Burkard, Guido},
  note={Article Number: 247701}
}
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