KOPS - Das Institutionelle Repositorium der Universität Konstanz

Charge-carrier-induced frequency renormalization, damping, and heating of vibrational modes in nanoscale junctions

Charge-carrier-induced frequency renormalization, damping, and heating of vibrational modes in nanoscale junctions

Zitieren

Dateien zu dieser Ressource

Dateien Größe Format Anzeige

Zu diesem Dokument gibt es keine Dateien.

KAASBJERG, Kristen, Tomas NOVOTNY, Abraham NITZAN, 2013. Charge-carrier-induced frequency renormalization, damping, and heating of vibrational modes in nanoscale junctions. In: Physical Review B. 88(20). ISSN 1098-0121. eISSN 1095-3795. Available under: doi: 10.1103/PhysRevB.88.201405

@article{Kaasbjerg2013Charg-26570, title={Charge-carrier-induced frequency renormalization, damping, and heating of vibrational modes in nanoscale junctions}, year={2013}, doi={10.1103/PhysRevB.88.201405}, number={20}, volume={88}, issn={1098-0121}, journal={Physical Review B}, author={Kaasbjerg, Kristen and Novotny, Tomas and Nitzan, Abraham} }

<rdf:RDF xmlns:dcterms="http://purl.org/dc/terms/" xmlns:dc="http://purl.org/dc/elements/1.1/" xmlns:rdf="http://www.w3.org/1999/02/22-rdf-syntax-ns#" xmlns:bibo="http://purl.org/ontology/bibo/" xmlns:dspace="http://digital-repositories.org/ontologies/dspace/0.1.0#" xmlns:foaf="http://xmlns.com/foaf/0.1/" xmlns:void="http://rdfs.org/ns/void#" xmlns:xsd="http://www.w3.org/2001/XMLSchema#" > <rdf:Description rdf:about="https://kops.uni-konstanz.de/rdf/resource/123456789/26570"> <dcterms:bibliographicCitation>Physical Review / B ; 88 (2013). - 201405(R)</dcterms:bibliographicCitation> <dcterms:isPartOf rdf:resource="https://kops.uni-konstanz.de/rdf/resource/123456789/41"/> <dcterms:title>Charge-carrier-induced frequency renormalization, damping, and heating of vibrational modes in nanoscale junctions</dcterms:title> <dspace:isPartOfCollection rdf:resource="https://kops.uni-konstanz.de/rdf/resource/123456789/41"/> <dc:creator>Novotny, Tomas</dc:creator> <dcterms:rights rdf:resource="http://nbn-resolving.org/urn:nbn:de:bsz:352-20140905103605204-4002607-1"/> <dc:creator>Kaasbjerg, Kristen</dc:creator> <dc:language>eng</dc:language> <dcterms:issued>2013</dcterms:issued> <bibo:uri rdf:resource="http://kops.uni-konstanz.de/handle/123456789/26570"/> <dc:contributor>Kaasbjerg, Kristen</dc:contributor> <dc:contributor>Nitzan, Abraham</dc:contributor> <dc:contributor>Novotny, Tomas</dc:contributor> <dcterms:available rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2014-03-05T12:21:25Z</dcterms:available> <dc:creator>Nitzan, Abraham</dc:creator> <foaf:homepage rdf:resource="http://localhost:8080/jspui"/> <dcterms:abstract xml:lang="eng">In nanoscale junctions the interaction between charge carriers and the local vibrations results in renormalization, damping, and heating of the vibrational modes. Here we formulate a nonequilibrium Green's function based theory to describe such effects. Studying a generic junction model with an off-resonant electronic level, we find a strong bias dependence of the frequency renormalization and vibrational damping accompanied by pronounced nonlinear vibrational heating in junctions with intermediate values of the coupling to the leads. Combining our theory with ab initio calculations, we furthermore show that the bias dependence of the Raman shifts and linewidths observed experimentally in an oligo(3)-phenylenevinylene (OPV3) junction [Ward et al., Nat. Nanotechnol. 6, 33 (2011)] may be explained by a combination of dynamic carrier screening and molecular charging.</dcterms:abstract> <dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2014-03-05T12:21:25Z</dc:date> <dc:rights>deposit-license</dc:rights> <void:sparqlEndpoint rdf:resource="http://localhost/fuseki/dspace/sparql"/> </rdf:Description> </rdf:RDF>

Das Dokument erscheint in:

KOPS Suche


Stöbern

Mein Benutzerkonto