KOPS - The Institutional Repository of the University of Konstanz

Toward far-field vibrational spectroscopy of single molecules at room temperature

Toward far-field vibrational spectroscopy of single molecules at room temperature

Cite This

Files in this item

Files Size Format View

There are no files associated with this item.

WINTERHALDER, Martin, Andreas ZUMBUSCH, Markus LIPPITZ, Michel ORRIT, 2011. Toward far-field vibrational spectroscopy of single molecules at room temperature. In: The Journal of Physical Chemistry B. 115(18), pp. 5425-5430. ISSN 1520-6106. eISSN 1520-5207. Available under: doi: 10.1021/jp109652s

@article{Winterhalder2011-05-12Towar-19304, title={Toward far-field vibrational spectroscopy of single molecules at room temperature}, year={2011}, doi={10.1021/jp109652s}, number={18}, volume={115}, issn={1520-6106}, journal={The Journal of Physical Chemistry B}, pages={5425--5430}, author={Winterhalder, Martin and Zumbusch, Andreas and Lippitz, Markus and Orrit, Michel} }

<rdf:RDF xmlns:dcterms="http://purl.org/dc/terms/" xmlns:dc="http://purl.org/dc/elements/1.1/" xmlns:rdf="http://www.w3.org/1999/02/22-rdf-syntax-ns#" xmlns:bibo="http://purl.org/ontology/bibo/" xmlns:dspace="http://digital-repositories.org/ontologies/dspace/0.1.0#" xmlns:foaf="http://xmlns.com/foaf/0.1/" xmlns:void="http://rdfs.org/ns/void#" xmlns:xsd="http://www.w3.org/2001/XMLSchema#" > <rdf:Description rdf:about="https://kops.uni-konstanz.de/rdf/resource/123456789/19304"> <dcterms:abstract xml:lang="eng">We propose a new scheme for the extraction of chemically sensitive vibrational information from a single fluorescent molecule at room temperature. Our approach is based on a three-photon fluorescence excitation scheme, with selectivity in the production of a vibrational population of the ground state. We estimate the expected signal in perturbation theory for a standard dye molecule, compare its magnitude qualitatively to noise and various background sources, and discuss the experimental realization of this scheme.</dcterms:abstract> <dc:creator>Orrit, Michel</dc:creator> <dc:date rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2012-05-16T06:34:21Z</dc:date> <void:sparqlEndpoint rdf:resource="http://localhost/fuseki/dspace/sparql"/> <dc:rights>terms-of-use</dc:rights> <dc:creator>Lippitz, Markus</dc:creator> <dc:contributor>Orrit, Michel</dc:contributor> <bibo:uri rdf:resource="http://kops.uni-konstanz.de/handle/123456789/19304"/> <dcterms:rights rdf:resource="https://kops.uni-konstanz.de/page/termsofuse"/> <dcterms:available rdf:datatype="http://www.w3.org/2001/XMLSchema#dateTime">2012-05-16T06:34:21Z</dcterms:available> <dcterms:isPartOf rdf:resource="https://kops.uni-konstanz.de/rdf/resource/123456789/29"/> <dcterms:title>Toward far-field vibrational spectroscopy of single molecules at room temperature</dcterms:title> <dspace:isPartOfCollection rdf:resource="https://kops.uni-konstanz.de/rdf/resource/123456789/29"/> <dc:contributor>Zumbusch, Andreas</dc:contributor> <dc:creator>Zumbusch, Andreas</dc:creator> <dcterms:issued>2011-05-12</dcterms:issued> <foaf:homepage rdf:resource="http://localhost:8080/jspui"/> <dc:creator>Winterhalder, Martin</dc:creator> <dc:language>eng</dc:language> <dc:contributor>Lippitz, Markus</dc:contributor> <dc:contributor>Winterhalder, Martin</dc:contributor> <dcterms:bibliographicCitation>Publ. in: The journal of physical chemistry B ; 115 (2011), 18. - S. 5425-5430</dcterms:bibliographicCitation> </rdf:Description> </rdf:RDF>

This item appears in the following Collection(s)

Search KOPS


Browse

My Account