Idealized glass transitions under pressure : Dynamics versus thermodynamics

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2008
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Physical Review Letters. 2008, 101(9). ISSN 0031-9007. Available under: doi: 10.1103/PhysRevLett.101.095701
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The interplay of slow dynamics and thermodynamic features of dense liquids is studied by examining how the glass transition changes depending on the presence or absence of Lennard-Jones-like attractions. Quite different thermodynamic behavior leaves the dynamics unchanged, with important consequences for high-pressure experiments on glassy liquids. Numerical results are obtained within mode-coupling theory (MCT), but the qualitative features are argued to hold more generally. A simple square-well model can be used to explain generic features found in experiment.

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ISO 690VOIGTMANN, Thomas, 2008. Idealized glass transitions under pressure : Dynamics versus thermodynamics. In: Physical Review Letters. 2008, 101(9). ISSN 0031-9007. Available under: doi: 10.1103/PhysRevLett.101.095701
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@article{Voigtmann2008Ideal-17112,
  year={2008},
  doi={10.1103/PhysRevLett.101.095701},
  title={Idealized glass transitions under pressure : Dynamics versus thermodynamics},
  number={9},
  volume={101},
  issn={0031-9007},
  journal={Physical Review Letters},
  author={Voigtmann, Thomas}
}
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