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Reply to Comment on 'Spin-selective reactions of radical pairs act as quantum measurements'

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2011

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Jones, Jonathan
Maeda, Kiminori
Hore, Peter

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http://nbn-resolving.de/urn:nbn:de:bsz:352-193080
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https://doi.org/10.1016/j.cplett.2011.04.022
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Chemical Physics Letters. 2011, 508(1-3), pp. 184-185. ISSN 0009-2614. Available under: doi: 10.1016/j.cplett.2011.04.022

Zusammenfassung

In his Comment on a recent paper by two of us Kominis claims that the recently proposed quantum measurement model for spin-selective reactions of radical pairs leads to ambiguous predictions in a simple case. Here we show that this claim is based on a confusion between the unreacted and unrecombined portions of the radical pairs, and to an incorrect interpretation of the improper density matrices used in both our model and the conventional Haberkorn model of such reactions. We further show that if this error is corrected then the supposed ambiguity is resolved.

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540 Chemie

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ISO 690JONES, Jonathan, Kiminori MAEDA, Ulrich STEINER, Peter HORE, 2011. Reply to Comment on 'Spin-selective reactions of radical pairs act as quantum measurements'. In: Chemical Physics Letters. 2011, 508(1-3), pp. 184-185. ISSN 0009-2614. Available under: doi: 10.1016/j.cplett.2011.04.022
BibTex
@article{Jones2011Reply-19308,
  year={2011},
  doi={10.1016/j.cplett.2011.04.022},
  title={Reply to Comment on 'Spin-selective reactions of radical pairs act as quantum measurements'},
  number={1-3},
  volume={508},
  issn={0009-2614},
  journal={Chemical Physics Letters},
  pages={184--185},
  author={Jones, Jonathan and Maeda, Kiminori and Steiner, Ulrich and Hore, Peter}
}
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    <dcterms:abstract xml:lang="eng">In his Comment on a recent paper by two of us Kominis claims that the recently proposed quantum measurement model for spin-selective reactions of radical pairs leads to ambiguous predictions in a simple case. Here we show that this claim is based on a confusion between the unreacted and unrecombined portions of the radical pairs, and to an incorrect interpretation of the improper density matrices used in both our model and the conventional Haberkorn model of such reactions. We further show that if this error is corrected then the supposed ambiguity is resolved.</dcterms:abstract>
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