Publikation:

Interfaces in Perovskite Solar Cells

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Datum

2017

Autor:innen

Garcia-Belmonte, Germà
Jose, Rajan
Mora-Sero, Ivan

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http://nbn-resolving.de/urn:nbn:de:bsz:352-2-b233ysieihl04
DOI (zitierfähiger Link)
https://doi.org/10.1002/aenm.201700623
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Open Access-Veröffentlichung
Open Access Green

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Physik: Publikationen
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Published

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Advanced Energy Materials. 2017, 7(22), 1700623. ISSN 1614-6832. eISSN 1614-6840. Available under: doi: 10.1002/aenm.201700623

Zusammenfassung

Rapid improvement in photoconversion efficiency (PCE) of solution processable organometallic hybrid halide based perovskite solar cells (PSCs) have taken the photovoltaic (PV) community with a surprise and has extended their application in other electronic devices such as light emitting diodes, photo detectors and batteries. Together with efforts to push the PCE of PSCs to record values >22% – now at par with that of crystalline silicon solar cells – origin of their PV action and underlying physical processes are also deeply investigated worldwide in diverse device configurations. A typical PSC consists of a perovskite film sandwiched between an electron and a hole selective contact thereby creating ESC/perovskite and perovskite/HSC interfaces, respectively. The selective contacts and their interfaces determine properties of perovskite layer and also control the performance, origin of PV action, open circuit voltage, device stability, and hysteresis in PSCs. Herein, we define ideal charge selective contacts, and provide an overview on how the choice of interfacing materials impacts charge accumulation, transport, transfer/recombination, band-alignment, and electrical stability in PSCs. We then discuss device related considerations such as morphology of the selective contacts (planar or mesoporous), energetics and electrical properties (insulating and conducting), and its chemical properties (organic vs inorganic). Finally, the outlook highlights key challenges and future directions for a commercially viable perovskite based PV technology.

Zusammenfassung in einer weiteren Sprache

Fachgebiet (DDC)
530 Physik

Schlagwörter

renewable energy; interfacial charge transfer; interface modification; interfacial defects in perovskite solar cells; hysteresis in perovskites

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ISO 690FAKHARUDDIN, Azhar, Lukas SCHMIDT-MENDE, Germà GARCIA-BELMONTE, Rajan JOSE, Ivan MORA-SERO, 2017. Interfaces in Perovskite Solar Cells. In: Advanced Energy Materials. 2017, 7(22), 1700623. ISSN 1614-6832. eISSN 1614-6840. Available under: doi: 10.1002/aenm.201700623
BibTex
@article{Fakharuddin2017-11Inter-40177,
  year={2017},
  doi={10.1002/aenm.201700623},
  title={Interfaces in Perovskite Solar Cells},
  number={22},
  volume={7},
  issn={1614-6832},
  journal={Advanced Energy Materials},
  author={Fakharuddin, Azhar and Schmidt-Mende, Lukas and Garcia-Belmonte, Germà and Jose, Rajan and Mora-Sero, Ivan},
  note={Article Number: 1700623}
}
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