Multiple Glassy State in a Simple Model System

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Date
2002
Authors
Pham, K. N.
Puertas, Antonio M.
Bergenholtz, Johan
Egelhaaf, Stefan Ulrich
Moussaid, A.
Pusey, Peter N.
Schofield, Andrew B.
Cates, Michael E.
Poon, Wilson C. K.
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Science ; 296 (2002). - pp. 104-106
Abstract
Experiments, theory, and simulation were used to study glass formation in a simple model system composed of hard spheres with short-range attraction (Òsticky hard spheresÓ). The experiments, using well-characterized colloids, revealed a reentrant glass transition line. Mode-coupling theory calculations and molecular dynamics simulations suggest that the reentrance is due to the existence of two qualitatively different glassy states: one dominated by repulsion (with structural arrest due to caging) and the other by attraction (with structural arrest due to bonding). This picture is consistent with a study of the particle dynamics in the colloid using dynamic light scattering.
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530 Physics
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ISO 690PHAM, K. N., Antonio M. PUERTAS, Johan BERGENHOLTZ, Stefan Ulrich EGELHAAF, A. MOUSSAID, Peter N. PUSEY, Andrew B. SCHOFIELD, Michael E. CATES, Matthias FUCHS, Wilson C. K. POON, 2002. Multiple Glassy State in a Simple Model System. In: Science. 296, pp. 104-106. Available under: doi: 10.1126/science.1068238
BibTex
@article{Pham2002Multi-4906,
  year={2002},
  doi={10.1126/science.1068238},
  title={Multiple Glassy State in a Simple Model System},
  volume={296},
  journal={Science},
  pages={104--106},
  author={Pham, K. N. and Puertas, Antonio M. and Bergenholtz, Johan and Egelhaaf, Stefan Ulrich and Moussaid, A. and Pusey, Peter N. and Schofield, Andrew B. and Cates, Michael E. and Fuchs, Matthias and Poon, Wilson C. K.}
}
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