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Purcell Effect and Photoluminescence Emission Enhancement of Individual CdSe/CdS/PMMA Nano Particles Coupled to Metallic Bullseye Resonators

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https://doi.org/10.1109/CLEOE-EQEC.2017.8087608
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2017 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO Europe-EQEC) : 25-29 June 2017. Piscataway, NJ: IEEE, 2017, EG_5_4. ISBN 978-1-5090-6736-7. Available under: doi: 10.1109/CLEOE-EQEC.2017.8087608

Zusammenfassung

Polymer-capped colloidal semiconductor quantum dots [1] offer a robust material system for time-resolved analysis and individual control of ultrafast charge carrier dynamics [2]. This goal necessitates a strong enhancement of light-matter interaction. In this work we demonstrate an efficient coupling of individual CdSe/CdS/PMMA quantum dots (QDs) to plasmonic resonators formed out of multiple concentric rings patterned in a 280-nm thick gold layer. Such a “bullseye” design allows for efficient manipulation of single QDs into the center of the antenna while imposing no polarization selectivity [3]. As a result, we achieve a dramatic increase of the photoluminescence (PL) emission intensity and the radiative decay rates due to the Purcell effect.

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2017 European Conference on Lasers and Electro-Optics and European Quantum Electronics Conference, 25. Juni 2017 - 29. Juni 2017, München
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ISO 690WERSCHLER, Florian, Benjamin LINDNER, Christopher HINZ, Tjaard DE ROO, Stefan MECKING, Denis V. SELETSKIY, Alfred LEITENSTORFER, 2017. Purcell Effect and Photoluminescence Emission Enhancement of Individual CdSe/CdS/PMMA Nano Particles Coupled to Metallic Bullseye Resonators. 2017 European Conference on Lasers and Electro-Optics and European Quantum Electronics Conference. München, 25. Juni 2017 - 29. Juni 2017. In: 2017 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO Europe-EQEC) : 25-29 June 2017. Piscataway, NJ: IEEE, 2017, EG_5_4. ISBN 978-1-5090-6736-7. Available under: doi: 10.1109/CLEOE-EQEC.2017.8087608
BibTex
@inproceedings{Werschler2017Purce-45681,
  year={2017},
  doi={10.1109/CLEOE-EQEC.2017.8087608},
  title={Purcell Effect and Photoluminescence Emission Enhancement of Individual CdSe/CdS/PMMA Nano Particles Coupled to Metallic Bullseye Resonators},
  isbn={978-1-5090-6736-7},
  publisher={IEEE},
  address={Piscataway, NJ},
  booktitle={2017 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO Europe-EQEC) : 25-29 June 2017},
  author={Werschler, Florian and Lindner, Benjamin and Hinz, Christopher and de Roo, Tjaard and Mecking, Stefan and Seletskiy, Denis V. and Leitenstorfer, Alfred},
  note={Article Number: EG_5_4}
}
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