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Real-time optical mapping of the dynamics of nonthermal electrons in thin gold films

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2012

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Della Valle, Giuseppe
Conforti, Matteo
Longhi, Stefano
Cerullo, Giulio

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http://nbn-resolving.de/urn:nbn:de:bsz:352-289540
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https://doi.org/10.1103/PhysRevB.86.155139
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Physical Review B. 2012, 86(15). ISSN 1098-0121. eISSN 0163-1829. Available under: doi: 10.1103/PhysRevB.86.155139

Zusammenfassung

We investigate the nonlinear optical response of thin gold films with an unprecedented combination of high temporal resolution (∼ 15 fs) and broad spectral coverage. We quantitatively model the data without free parameters using an extended version of the two-temperature model. Our combined experimental and theoretical approach allows tracking the evolution from a purely nonthermal electron distribution towards a fully thermalized one. These results pose the basis for better understanding of light-matter interaction in metals on the ultrafast time scale.

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ISO 690DELLA VALLE, Giuseppe, Matteo CONFORTI, Stefano LONGHI, Giulio CERULLO, Daniele BRIDA, 2012. Real-time optical mapping of the dynamics of nonthermal electrons in thin gold films. In: Physical Review B. 2012, 86(15). ISSN 1098-0121. eISSN 0163-1829. Available under: doi: 10.1103/PhysRevB.86.155139
BibTex
@article{DellaValle2012Realt-28954,
  year={2012},
  doi={10.1103/PhysRevB.86.155139},
  title={Real-time optical mapping of the dynamics of nonthermal electrons in thin gold films},
  number={15},
  volume={86},
  issn={1098-0121},
  journal={Physical Review B},
  author={Della Valle, Giuseppe and Conforti, Matteo and Longhi, Stefano and Cerullo, Giulio and Brida, Daniele}
}
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