Publikation: A comparison of photoelectron spectroscopy and two-photon ionization spectroscopy : excited states of Au2, Au3, and Au4
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Photoelectron spectra of Au - n with n=2–4 are reported. Due to the relatively high photon energy used in our experiment (hnu=6.424 eV) and the energy resolution of about 50 meV, various transitions into excited states of the neutral clusters are resolved. It is demonstrated that photoelectron spectra can serve as a map of the electronic states of a cluster, while the high resolution of the resonant two-photon ionization (R2PI) method gains information about the symmetry of the states. The comparison with similar data of Agn- clusters indicates the influence of relativistic effects and the large spin–orbit splitting for Au.
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HANDSCHUH, Haiko, Gerd GANTEFÖR, Paul S. BECHTHOLD, Wolfgang EBERHARDT, 1994. A comparison of photoelectron spectroscopy and two-photon ionization spectroscopy : excited states of Au2, Au3, and Au4. In: Journal of Chemical Physics. 1994, 100(10), pp. 7093-7100. Available under: doi: 10.1063/1.467267BibTex
@article{Handschuh1994compa-9089, year={1994}, doi={10.1063/1.467267}, title={A comparison of photoelectron spectroscopy and two-photon ionization spectroscopy : excited states of Au2, Au3, and Au4}, number={10}, volume={100}, journal={Journal of Chemical Physics}, pages={7093--7100}, author={Handschuh, Haiko and Ganteför, Gerd and Bechthold, Paul S. and Eberhardt, Wolfgang} }
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