28-fs electron pulses for atomic-scale diffraction

Gliserin, Alexander; Walbran, Matthew; Krausz, Ferenc; Baum, Peter

28-fs electron pulses for atomic-scale diffraction

Dateien

Gliserin_2-1lj5u6gizvurk1.pdfGröße: 693.71 KBDownloads: 130

Datum

2015

Autor:innen

Gliserin, Alexander

Walbran, Matthew

Krausz, Ferenc

Baum, Peter

URI (zitierfähiger Link)

http://nbn-resolving.de/urn:nbn:de:bsz:352-2-1lj5u6gizvurk1

Link zur Lizenz

Urheberrechtlich geschützt

Open Access-Veröffentlichung

Open Access Green

Sammlungen

Physik

Publikationstyp

Preprint

Publikationsstatus

Published

Zusammenfassung

Visualizing the rearrangement of atoms in a wide range of molecular and condensed-matter systems requires resolving picometer displacements on a ten-femtosecond time scale. Here we demonstrate the compression of single-electron pulses with a de Broglie wavelength of 0.08 ångström to a duration of 28±5 femtoseconds (full width at half maximum) or 12±2 femtoseconds (standard deviation), substantially shorter than any laser pulses involved. Atomic resolution diffraction from a complex organic molecule is obtained with good signalto- noise ratio within a data acquisition period of minutes. The electron-laser timing is found to be stable within 5 fs (standard deviation) over several hours, allowing pump-probe diffraction at repetitive excitation. These measurements show the feasibility of laserpump/ electron-probe scans that can resolve the fastest atomic motions relevant in reversible condensed matter transformations and organic chemistry.

Fachgebiet (DDC)

530 Physik

Zitieren

ISO 690

GLISERIN, Alexander, Matthew WALBRAN, Ferenc KRAUSZ, Peter BAUM, 2015. 28-fs electron pulses for atomic-scale diffraction

BibTex

@unpublished{Gliserin2015elect-51898,
  year={2015},
  title={28-fs electron pulses for atomic-scale diffraction},
  author={Gliserin, Alexander and Walbran, Matthew and Krausz, Ferenc and Baum, Peter},
  note={Published version: https://dx.doi.org/10.1038/ncomms9723}
}

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Kommentar zur Publikation

Published version: https://dx.doi.org/10.1038/ncomms9723

Universitätsbibliographie

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