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Direct evidence of Rabi oscillations and antiresonance in a strongly coupled organic microcavity

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2015

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Rajendran, Sai K.
De Sio, Antonietta
Sommer, Ephraim
Vogelgesang, Ralf
Coles, David
Lidzey, David G.
Cerullo, Giulio
Lienau, Christoph
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https://doi.org/10.1103/PhysRevB.91.201305
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Physical Review B. 2015, 91(20), 201305. ISSN 1098-0121. eISSN 1095-3795. Available under: doi: 10.1103/PhysRevB.91.201305

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We report the direct observation of 30-fs period Rabi oscillations between excitons and cavity photons in a strongly coupled J-aggregate microcavity by means of time-resolved up-conversion and spectral interferometry measurements. The time structure of the transmitted electric field, measured by linear spectral interferometry, shows pronounced ultrafast beats. Its spectral phase reveals a distinct signature caused by destructive interference between the coherent drive and the field radiated by the exciton. This antiresonance selectively probes the uncoupled exciton excitation, and its observation uncovers the coherent and ultrafast exchange of energy between the optically excited cavity and the J-aggregate excitons, as confirmed by transfer matrix calculations.

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ISO 690RAJENDRAN, Sai K., Wei WANG, Daniele BRIDA, Antonietta DE SIO, Ephraim SOMMER, Ralf VOGELGESANG, David COLES, David G. LIDZEY, Giulio CERULLO, Christoph LIENAU, Tersilla VIRGILI, 2015. Direct evidence of Rabi oscillations and antiresonance in a strongly coupled organic microcavity. In: Physical Review B. 2015, 91(20), 201305. ISSN 1098-0121. eISSN 1095-3795. Available under: doi: 10.1103/PhysRevB.91.201305
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@article{Rajendran2015Direc-31280,
  year={2015},
  doi={10.1103/PhysRevB.91.201305},
  title={Direct evidence of Rabi oscillations and antiresonance in a strongly coupled organic microcavity},
  number={20},
  volume={91},
  issn={1098-0121},
  journal={Physical Review B},
  author={Rajendran, Sai K. and Wang, Wei and Brida, Daniele and De Sio, Antonietta and Sommer, Ephraim and Vogelgesang, Ralf and Coles, David and Lidzey, David G. and Cerullo, Giulio and Lienau, Christoph and Virgili, Tersilla},
  note={Article Number: 201305}
}
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