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Dual redox-active porous polyimides as high performance and versatile electrode material for next-generation batteries

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2023

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Goujon, Nicolas
Lahnsteiner, Marianne
Moura, Hipassia M.
Mantione, Daniele
Mecerreyes, David

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Materials Horizons. Royal Society of Chemistry (RSC). 2023, 10(3), pp. 967-976. ISSN 2051-6347. eISSN 2051-6355. Available under: doi: 10.1039/d2mh01335e

Zusammenfassung

Energy storage will be a primordial actor of the ecological transition initiated in the energy and transport sectors. As such, innovative approaches to design high-performance electrode materials are crucial for the development of the next generation of batteries. Herein, a novel dual redox-active and porous polyimide network (MTA-MPT), based on mellitic trianhydride (MTA) and 3,7-diamino-N-methylphenothiazine (MPT) monomers, is proposed for applications in both high energy density lithium batteries and symmetric all-organic batteries. The MTA-MPT porous polyimide was synthesized using a novel environmentally-friendly hydrothermal polymerization method. Rooted in its dual redox proprieties, the MTA-MPT porous polyimide exhibits a high theoretical capacity making it a very attractive cathode material for high energy density battery applications. The cycling performance of this novel electrode material was assessed in both high energy density lithium batteries and light-weight symmetric all-organic batteries, displaying excellent rate capability and long-term cycling stability.

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ISO 690GOUJON, Nicolas, Marianne LAHNSTEINER, Daniel Alonso CERRÓN INFANTES, Hipassia M. MOURA, Daniele MANTIONE, Miriam M. UNTERLASS, David MECERREYES, 2023. Dual redox-active porous polyimides as high performance and versatile electrode material for next-generation batteries. In: Materials Horizons. Royal Society of Chemistry (RSC). 2023, 10(3), pp. 967-976. ISSN 2051-6347. eISSN 2051-6355. Available under: doi: 10.1039/d2mh01335e
BibTex
@article{Goujon2023redox-66389,
  year={2023},
  doi={10.1039/d2mh01335e},
  title={Dual redox-active porous polyimides as high performance and versatile electrode material for next-generation batteries},
  number={3},
  volume={10},
  issn={2051-6347},
  journal={Materials Horizons},
  pages={967--976},
  author={Goujon, Nicolas and Lahnsteiner, Marianne and Cerrón Infantes, Daniel Alonso and Moura, Hipassia M. and Mantione, Daniele and Unterlass, Miriam M. and Mecerreyes, David}
}
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