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Light scattering spectroscopy of the liquid-glass transition : comparison with idealized and extended mode coupling theory

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1993

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Cummins, Herman Z.
Du, W. M.
Götze, Wolfgang
Latz, Arnulf
Li, G.
Tao, N. J.

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Physica / A [Statistical Mechanics]. 1993, 201, pp. 207-222. Available under: doi: 10.1016/0378-4371(93)90417-3

Zusammenfassung

Light scattering experiments were performed on several fragile glass-forming materials at temperatures ranging from above the melting temperature Tm to below the calorimetric glass transition temperature T in the frequency range 0.2 GHz to 4000 GHz. The experimental susceptibility spectra x(w) exhibit both the form and the scaling properties predicted by the idealized mode coupling theory. At low frequencies and temperatures the spectra deviate from the predictions due to the neglect of ergodicity-restoring activated transport (hopping) processes. We have therefore reanalyzed the data using the extended version of the theory, including activated transport.

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530 Physik

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ISO 690CUMMINS, Herman Z., W. M. DU, Matthias FUCHS, Wolfgang GÖTZE, Arnulf LATZ, G. LI, N. J. TAO, 1993. Light scattering spectroscopy of the liquid-glass transition : comparison with idealized and extended mode coupling theory. In: Physica / A [Statistical Mechanics]. 1993, 201, pp. 207-222. Available under: doi: 10.1016/0378-4371(93)90417-3
BibTex
@article{Cummins1993Light-5038,
  year={1993},
  doi={10.1016/0378-4371(93)90417-3},
  title={Light scattering spectroscopy of the liquid-glass transition : comparison with idealized and extended mode coupling theory},
  volume={201},
  journal={Physica / A [Statistical Mechanics]},
  pages={207--222},
  author={Cummins, Herman Z. and Du, W. M. and Fuchs, Matthias and Götze, Wolfgang and Latz, Arnulf and Li, G. and Tao, N. J.}
}
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