Force-induced diffusion in microrheology
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We investigate the force-induced diffusive motion of a tracer particle inside a glass-forming suspension when a strong external force is applied to the probe (active nonlinear microrheology). A schematic model of mode-coupling theory introduced recently is extended to describe the transient dynamics of the probe particle, and used to analyze recent molecular-dynamics simulation data. The model describes non-trivial transient displacements of the probe before a steady-state velocity is reached. The external force also induces diffusive motion in the direction perpendicular to its axis. We address the relation between the transverse diffusion coefficient D⊥ and the force-dependent nonlinear friction coefficient ζ. Non-diffusive fluctuations in the direction of the force are seen at long times in the MD simulation, while the model describes cross-over to long-time diffusion.
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HARR, Christian, D. WINTER, Jürgen HORBACH, Matthias FUCHS, Thomas VOIGTMANN, 2012. Force-induced diffusion in microrheology. In: Journal of Physics: Condensed Matter. 2012, 24(46), 464105. ISSN 0953-8984. eISSN 1361-648X. Available under: doi: 10.1088/0953-8984/24/46/464105BibTex
@article{Harr2012-11-21Force-25432, year={2012}, doi={10.1088/0953-8984/24/46/464105}, title={Force-induced diffusion in microrheology}, number={46}, volume={24}, issn={0953-8984}, journal={Journal of Physics: Condensed Matter}, author={Harr, Christian and Winter, D. and Horbach, Jürgen and Fuchs, Matthias and Voigtmann, Thomas}, note={Article Number: 464105} }
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