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Unidirectional hopping transport of interacting particles on a finite chain

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2010

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Einax, Mario
Solomon, Gemma C.

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https://doi.org/10.1063/1.3463000
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http://arxiv.org/abs/1005.0864

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The Journal of Chemical Physics. American Institute of Physics (AIP). 2010, 133(5), 054102. ISSN 0021-9606. eISSN 1089-7690. Available under: doi: 10.1063/1.3463000

Zusammenfassung

Particle transport through an open, discrete one-dimensional channel against a mechanical or chemical bias is analyzed within a master equation approach. The channel, externally driven by time-dependent site energies, allows multiple occupation due to the coupling to reservoirs. Performance criteria and optimization of active transport in a two-site channel are discussed as a function of reservoir chemical potentials, the load potential, interparticle interaction strength, driving mode, and driving period. Our results, derived from exact rate equations, are used in addition to test a previously developed time-dependent density functional theory, suggesting a wider applicability of that method in investigations of many particle systems far from equilibrium.

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ISO 690EINAX, Mario, Gemma C. SOLOMON, Wolfgang DIETERICH, Abraham NITZAN, 2010. Unidirectional hopping transport of interacting particles on a finite chain. In: The Journal of Chemical Physics. American Institute of Physics (AIP). 2010, 133(5), 054102. ISSN 0021-9606. eISSN 1089-7690. Available under: doi: 10.1063/1.3463000
BibTex
@article{Einax2010-08-07Unidi-51595,
  year={2010},
  doi={10.1063/1.3463000},
  title={Unidirectional hopping transport of interacting particles on a finite chain},
  number={5},
  volume={133},
  issn={0021-9606},
  journal={The Journal of Chemical Physics},
  author={Einax, Mario and Solomon, Gemma C. and Dieterich, Wolfgang and Nitzan, Abraham},
  note={Article Number: 054102}
}
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