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Self-consistent rate theory for submonolayer surface growth of multicomponent systems

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2014

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Einax, Mario
Maass, Philipp
Dieterich, Wolfgang

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https://doi.org/10.1103/PhysRevB.90.035441
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Physical Review B. 2014, 90(3), 035441. ISSN 0163-1829. eISSN 1095-3795. Available under: doi: 10.1103/PhysRevB.90.035441

Zusammenfassung

The self-consistent rate theory for surface growth in the submonolayer regime is generalized from mono- to multicomponent systems, which are formed by codeposition of different types of atoms or molecules. The theory requires the introduction of pair density distributions to enable a symmetric treatment of reactions among different species. The approach is explicitly developed for binary systems and tested against kinetic Monte Carlo simulations. Using a reduced set of rate equations, only a few differential equations need to be solved to obtain good quantitative predictions for island and adatom densities, as well as densities of unstable clusters.

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ISO 690EINAX, Mario, Philipp MAASS, Wolfgang DIETERICH, 2014. Self-consistent rate theory for submonolayer surface growth of multicomponent systems. In: Physical Review B. 2014, 90(3), 035441. ISSN 0163-1829. eISSN 1095-3795. Available under: doi: 10.1103/PhysRevB.90.035441
BibTex
@article{Einax2014Selfc-29262,
  year={2014},
  doi={10.1103/PhysRevB.90.035441},
  title={Self-consistent rate theory for submonolayer surface growth of multicomponent systems},
  number={3},
  volume={90},
  issn={0163-1829},
  journal={Physical Review B},
  author={Einax, Mario and Maass, Philipp and Dieterich, Wolfgang},
  note={Article Number: 035441}
}
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