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Marangoni spreading and contracting three-component droplets on completely wetting surfaces

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2022

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Baumgartner, Dieter A.
Shiri, Samira
Sinha, Shayandev
Cira, Nate J.

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Proceedings of the National Academy of Sciences of the United States of America (PNAS). Proceedings of the National Academy of Sciences. 2022, 119(19), e2120432119. ISSN 0027-8424. eISSN 1091-6490. Available under: doi: 10.1073/pnas.2120432119

Zusammenfassung

When a droplet comes in contact with a completely wetting surface, the liquid typically spreads until it covers the entire substrate. However, nonuniform evaporation of a multicomponent droplet can generate surface tension gradients that alter this behavior. Here, we explore the rich dynamics of fully miscible, three-component droplets composed of water, ethanol, and propylene glycol on completely wetting glass substrates. These droplets initially spread rapidly but then stop and contract. We experimentally and theoretically investigate this behavior throughout the ternary parameter space at different relative humidities. Evaporation changes the composition of the droplet over space and time, resulting in a reversal of Marangoni flows that ultimately determines the dynamic droplet shape. We illustrate the utility of such dynamics by collecting, aggregating, and removing contaminants from a 4-cm2 area using a single µL-scale droplet.

Zusammenfassung in einer weiteren Sprache

Fachgebiet (DDC)
530 Physik

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surface wetting, Marangoni stress, multicomponent droplet, surface cleaning, evaporating droplet

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ISO 690BAUMGARTNER, Dieter A., Samira SHIRI, Shayandev SINHA, Stefan KARPITSCHKA, Nate J. CIRA, 2022. Marangoni spreading and contracting three-component droplets on completely wetting surfaces. In: Proceedings of the National Academy of Sciences of the United States of America (PNAS). Proceedings of the National Academy of Sciences. 2022, 119(19), e2120432119. ISSN 0027-8424. eISSN 1091-6490. Available under: doi: 10.1073/pnas.2120432119
BibTex
@article{Baumgartner2022Maran-67206,
  year={2022},
  doi={10.1073/pnas.2120432119},
  title={Marangoni spreading and contracting three-component droplets on completely wetting surfaces},
  number={19},
  volume={119},
  issn={0027-8424},
  journal={Proceedings of the National Academy of Sciences of the United States of America (PNAS)},
  author={Baumgartner, Dieter A. and Shiri, Samira and Sinha, Shayandev and Karpitschka, Stefan and Cira, Nate J.},
  note={Article Number: e2120432119}
}
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