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Diversity-Oriented Synthesis of Steviol Glycosides

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2018

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Qiao, Zhi
Liu, Hui
Sui, Jing-Jing
Liao, Jin-Xi
Tu, Yuan-Hong
Sun, Jian-Song

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https://doi.org/10.1021/acs.joc.8b01274
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The Journal of Organic Chemistry. 2018, 83(19), pp. 11480-11492. ISSN 0022-3263. eISSN 1520-6904. Available under: doi: 10.1021/acs.joc.8b01274

Zusammenfassung

With cheap and easily available mixtures of steviol glycosides as starting materials, a practical method for steviol acquisition has been developed, on the basis of which a facile, diversity-oriented, and economic protocol for the synthesis of structurally defined steviol glycosides was established. The novel approach is featured by the highly efficient glycosylation of sterically hindered and acid-sensitive steviol via orchestrated application of Yu glycosylation, Schmidt glycosylation, and PTC glycosylation. Hence, these high-intensity sweeteners and potential lead compounds for drug development are now readily accessible.

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ISO 690QIAO, Zhi, Hui LIU, Jing-Jing SUI, Jin-Xi LIAO, Yuan-Hong TU, Richard R. SCHMIDT, Jian-Song SUN, 2018. Diversity-Oriented Synthesis of Steviol Glycosides. In: The Journal of Organic Chemistry. 2018, 83(19), pp. 11480-11492. ISSN 0022-3263. eISSN 1520-6904. Available under: doi: 10.1021/acs.joc.8b01274
BibTex
@article{Qiao2018-10-05Diver-43930,
  year={2018},
  doi={10.1021/acs.joc.8b01274},
  title={Diversity-Oriented Synthesis of Steviol Glycosides},
  number={19},
  volume={83},
  issn={0022-3263},
  journal={The Journal of Organic Chemistry},
  pages={11480--11492},
  author={Qiao, Zhi and Liu, Hui and Sui, Jing-Jing and Liao, Jin-Xi and Tu, Yuan-Hong and Schmidt, Richard R. and Sun, Jian-Song}
}
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