Toward far-field vibrational spectroscopy of single molecules at room temperature

dc.contributor.authorWinterhalder, Martin
dc.contributor.authorZumbusch, Andreas
dc.contributor.authorLippitz, Markusdeu
dc.contributor.authorOrrit, Micheldeu
dc.date.accessioned2012-05-16T06:34:21Zdeu
dc.date.available2012-05-16T06:34:21Zdeu
dc.date.issued2011-05-12
dc.description.abstractWe propose a new scheme for the extraction of chemically sensitive vibrational information from a single fluorescent molecule at room temperature. Our approach is based on a three-photon fluorescence excitation scheme, with selectivity in the production of a vibrational population of the ground state. We estimate the expected signal in perturbation theory for a standard dye molecule, compare its magnitude qualitatively to noise and various background sources, and discuss the experimental realization of this scheme.eng
dc.description.versionpublished
dc.identifier.citationPubl. in: The journal of physical chemistry B ; 115 (2011), 18. - S. 5425-5430deu
dc.identifier.doi10.1021/jp109652sdeu
dc.identifier.pmid21381637
dc.identifier.urihttp://kops.uni-konstanz.de/handle/123456789/19304
dc.language.isoengdeu
dc.legacy.dateIssued2012-05-16deu
dc.rightsterms-of-usedeu
dc.rights.urihttps://rightsstatements.org/page/InC/1.0/deu
dc.subject.ddc540deu
dc.titleToward far-field vibrational spectroscopy of single molecules at room temperatureeng
dc.typeJOURNAL_ARTICLEdeu
dspace.entity.typePublication
kops.citation.bibtex
@article{Winterhalder2011-05-12Towar-19304,
  year={2011},
  doi={10.1021/jp109652s},
  title={Toward far-field vibrational spectroscopy of single molecules at room temperature},
  number={18},
  volume={115},
  issn={1520-6106},
  journal={The Journal of Physical Chemistry B},
  pages={5425--5430},
  author={Winterhalder, Martin and Zumbusch, Andreas and Lippitz, Markus and Orrit, Michel}
}
kops.citation.iso690WINTERHALDER, Martin, Andreas ZUMBUSCH, Markus LIPPITZ, Michel ORRIT, 2011. Toward far-field vibrational spectroscopy of single molecules at room temperature. In: The Journal of Physical Chemistry B. 2011, 115(18), pp. 5425-5430. ISSN 1520-6106. eISSN 1520-5207. Available under: doi: 10.1021/jp109652sdeu
kops.citation.iso690WINTERHALDER, Martin, Andreas ZUMBUSCH, Markus LIPPITZ, Michel ORRIT, 2011. Toward far-field vibrational spectroscopy of single molecules at room temperature. In: The Journal of Physical Chemistry B. 2011, 115(18), pp. 5425-5430. ISSN 1520-6106. eISSN 1520-5207. Available under: doi: 10.1021/jp109652seng
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kops.sourcefieldThe Journal of Physical Chemistry B. 2011, <b>115</b>(18), pp. 5425-5430. ISSN 1520-6106. eISSN 1520-5207. Available under: doi: 10.1021/jp109652sdeu
kops.sourcefield.plainThe Journal of Physical Chemistry B. 2011, 115(18), pp. 5425-5430. ISSN 1520-6106. eISSN 1520-5207. Available under: doi: 10.1021/jp109652sdeu
kops.sourcefield.plainThe Journal of Physical Chemistry B. 2011, 115(18), pp. 5425-5430. ISSN 1520-6106. eISSN 1520-5207. Available under: doi: 10.1021/jp109652seng
kops.submitter.emaillarysa.herasymova@uni-konstanz.dedeu
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source.periodicalTitleThe Journal of Physical Chemistry B

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