Publikation:

Toward far-field vibrational spectroscopy of single molecules at room temperature

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2011

Autor:innen

Winterhalder, Martin
Zumbusch, Andreas
Lippitz, Markus
Orrit, Michel

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http://nbn-resolving.de/urn:nbn:de:bsz:352-193046
DOI (zitierfähiger Link)
https://doi.org/10.1021/jp109652s
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Chemie: Publikationen
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The Journal of Physical Chemistry B. 2011, 115(18), pp. 5425-5430. ISSN 1520-6106. eISSN 1520-5207. Available under: doi: 10.1021/jp109652s

Zusammenfassung

We propose a new scheme for the extraction of chemically sensitive vibrational information from a single fluorescent molecule at room temperature. Our approach is based on a three-photon fluorescence excitation scheme, with selectivity in the production of a vibrational population of the ground state. We estimate the expected signal in perturbation theory for a standard dye molecule, compare its magnitude qualitatively to noise and various background sources, and discuss the experimental realization of this scheme.

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540 Chemie

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ISO 690WINTERHALDER, Martin, Andreas ZUMBUSCH, Markus LIPPITZ, Michel ORRIT, 2011. Toward far-field vibrational spectroscopy of single molecules at room temperature. In: The Journal of Physical Chemistry B. 2011, 115(18), pp. 5425-5430. ISSN 1520-6106. eISSN 1520-5207. Available under: doi: 10.1021/jp109652s
BibTex
@article{Winterhalder2011-05-12Towar-19304,
  year={2011},
  doi={10.1021/jp109652s},
  title={Toward far-field vibrational spectroscopy of single molecules at room temperature},
  number={18},
  volume={115},
  issn={1520-6106},
  journal={The Journal of Physical Chemistry B},
  pages={5425--5430},
  author={Winterhalder, Martin and Zumbusch, Andreas and Lippitz, Markus and Orrit, Michel}
}
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    <dcterms:abstract xml:lang="eng">We propose a new scheme for the extraction of chemically sensitive vibrational information from a single fluorescent molecule at room temperature. Our approach is based on a three-photon fluorescence excitation scheme, with selectivity in the production of a vibrational population of the ground state. We estimate the expected signal in perturbation theory for a standard dye molecule, compare its magnitude qualitatively to noise and various background sources, and discuss the experimental realization of this scheme.</dcterms:abstract>
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