Dual-oscillator infrared electro-optic sampling with attosecond precision

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2024
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Weigel, Alexander
Jacob, Philip
Schweinberger, Wolfgang
Huber, Marinus
Trubetskov, Michael
Karandušovský, Patrik
Hofer, Christina
Pupeza, Ioachim
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Deutsche Forschungsgemeinschaft (DFG): EXC 2051
Deutsche Forschungsgemeinschaft (DFG): 390713860
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Optica. Optica Publishing. 2024, 11(5), S. 726-735. eISSN 2334-2536. Verfügbar unter: doi: 10.1364/optica.515708
Zusammenfassung

Electro-optic sampling of infrared electric fields has set sensitivity and dynamic-range records in broadband molecular vibrational spectroscopy. Yet, in these works, the 1-second-scale single-trace acquisition time leads to intra-scan noise accumulation and restricts the throughput in measurements of multiple samples and of dynamic processes. We present a dual-laser-oscillator approach capturing 2800 mid-infrared waveforms per second by scanning the relative delay between the sampled waveform and the gate pulses using a modulated repetition-frequency lock. The new technique of electro-optic delay tracking (EODT) provides delay calibration with down to few-attosecond precision and provides a general route to high-precision dual-oscillator spectroscopy with picosecond delay ranges. Our work has immediate applications in, e.g., precision electric-field metrology and high-speed biosensing.

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ISO 690WEIGEL, Alexander, Philip JACOB, Wolfgang SCHWEINBERGER, Marinus HUBER, Michael TRUBETSKOV, Patrik KARANDUŠOVSKÝ, Christina HOFER, Philipp SULZER, Alfred LEITENSTORFER, Ioachim PUPEZA, 2024. Dual-oscillator infrared electro-optic sampling with attosecond precision. In: Optica. Optica Publishing. 2024, 11(5), S. 726-735. eISSN 2334-2536. Verfügbar unter: doi: 10.1364/optica.515708
BibTex
@article{Weigel2024-05-20Dualo-70139,
  year={2024},
  doi={10.1364/optica.515708},
  title={Dual-oscillator infrared electro-optic sampling with attosecond precision},
  number={5},
  volume={11},
  journal={Optica},
  pages={726--735},
  author={Weigel, Alexander and Jacob, Philip and Schweinberger, Wolfgang and Huber, Marinus and Trubetskov, Michael and Karandušovský, Patrik and Hofer, Christina and Sulzer, Philipp and Leitenstorfer, Alfred and Pupeza, Ioachim}
}
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