Complex nature of exchange splitting in oxide ferromagnets : A spin-resolved photoemission study of EuO
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The electronic structure of the ferromagnetic semiconductor EuO is investigated by means of spin- and angle-resolved photoemission spectroscopy and density functional theory. Our spin-resolved data reveals that, while the macroscopic magnetization of the sample vanishes at the Curie temperature TC, the experimentally-determined exchange splitting of the O 2p band persists at least up to TC if the picture of fluctuating spin-blocks is assumed. We discuss possible temperature-related spectral changes by analyzing ferromagnetic and antiferromagnetic phases, directional effect due to spin orbit coupling, as well as effects due to sample aging. Our calculations with a Hubbard U term reveal a complex nature of the local exchange splitting on the oxygen site and in conduction bands, shining a new light on the interpretation of previous optical and photoemission spectroscopic results.
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HEIDER, Tristan, Tim GERBER, Okan KÖKSAL, Markus ESCHBACH, Ewa MLYNCZAK, Patrick LÖMKER, Pika GOSPODARIC, Mathias GEHLMANN, Lukasz PLUCINSKI, Martina MÜLLER, 2020. Complex nature of exchange splitting in oxide ferromagnets : A spin-resolved photoemission study of EuOBibTex
@unpublished{Heider2020Compl-53584, year={2020}, title={Complex nature of exchange splitting in oxide ferromagnets : A spin-resolved photoemission study of EuO}, author={Heider, Tristan and Gerber, Tim and Köksal, Okan and Eschbach, Markus and Mlynczak, Ewa and Lömker, Patrick and Gospodaric, Pika and Gehlmann, Mathias and Plucinski, Lukasz and Müller, Martina} }
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